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Design of Orthogonal Reactions in Holographic Polymer Materials
- ACTA POLYMERICA SINICA Vol. 53, Issue 7, Pages: 722-736(2022)
- 作者机构：
华中科技大学化学与化工学院 能量转换与存储材料化学教育部重点实验室 武汉 430074
- 作者简介：
- 基金信息：
DOI：10.11777/j.issn1000-3304.2022.22053
CLC：Published：20 July 2022，
Published Online：01 June 2022，
Received：25 February 2022，
Accepted：19 April 2022
- 稿件说明：
移动端阅览
郭红喜,姚铭,赵晔等.全息高分子材料的正交反应设计[J].高分子学报,2022,53(07):722-736.
Guo Hong-xi,Yao Ming,Zhao Ye,et al.Design of Orthogonal Reactions in Holographic Polymer Materials[J].ACTA POLYMERICA SINICA,2022,53(07):722-736.
郭红喜,姚铭,赵晔等.全息高分子材料的正交反应设计[J].高分子学报,2022,53(07):722-736. DOI： 10.11777/j.issn1000-3304.2022.22053.
Guo Hong-xi,Yao Ming,Zhao Ye,et al.Design of Orthogonal Reactions in Holographic Polymer Materials[J].ACTA POLYMERICA SINICA,2022,53(07):722-736. DOI： 10.11777/j.issn1000-3304.2022.22053.
摘要
全息高分子材料通常是指基于相干激光技术制备，能够同时存储光波振幅、相位等全部信息的结构有序高分子材料，在裸眼三维显示、增强现实、高端防伪、高密度数据存储等高新技术领域具有重要应用价值. 高性能化与多功能化是全息高分子材料的发展方向，正交反应设计提供了有效途径. 本文简要介绍正交反应的概念、设计原理及在高分子材料先进制造中的应用，重点论述正交反应设计对于优化全息高分子材料加工工艺、提高折射率调制度和光栅衍射效率、降低雾度、抑制聚合反应引起的体积收缩、增加全息数据存储容量及构筑全息/发光双重图像功能新材料的重要性. 为获得高性能多功能全息高分子材料，亟需发展更加丰富的正交反应体系.
Abstract
Holographic polymer materials usually refer to structurally ordered polymer materials
which can store the whole information of light including the amplitude and phase upon laser interference. They have exhibited transformative potential for high-tech applications such as naked-eye recognizable three-dimensional display
augmented reality
high-security level anticounterfeiting and high-density data storage. With the development of these high-tech fields
it is highly desired to boost the performance and functionalities of holographic polymer materials. Toward this end
mediating reaction orthogonality can be an effective approach. Starting from the concept and design principle of orthogonal reactions
in this minireview
recent progresses of advanced manufacturing based on orthogonal reactions are highlighted. Furthermore
the significance of orthogonal reactions in holographic polymer materials are discussed in detail
for instances
to optimize material processing
to increase the refractive index modulation and grating diffraction efficiency
to decrease haze
to reduce volumetric shrinkage during polymerization
to increase the data storage capacity
and to non-interferingly integrate holographic and emissive dual images. Yet
new orthogonal reaction systems are still highly awaited to design high performance and multifunctional holographic polymer materials.
关键词
全息光聚合物正交反应先进制造
Keywords
HolographyPhotopolymerOrthogonal reactionsAdvanced manufacturing
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