Recent Advancements in Stretchable Polymer Optoelectronics

Si-yi Wang; Wen-kai Zhong; Fei Huang

doi:10.11777/j.issn1000-3304.2024.24131

您当前的位置：

首页 >

文章列表页 >

Recent Advancements in Stretchable Polymer Optoelectronics

Review | 更新时间：2024-11-26

- Recent Advancements in Stretchable Polymer Optoelectronics
- Acta Polymerica Sinica Vol. 55, Issue 9, Pages: 1091-1110(2024)
- 作者机构：
  
  华南理工大学高分子光电材料与器件研究所发光材料与器件国家重点实验室广州 510640
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2024.24131
  CLC：
- Published：20 September 2024，
  
  Published Online：12 July 2024，
  
  Received：07 May 2024，
  
  Accepted：23 May 2024
- 稿件说明：
移动端阅览
王思怡, 钟文楷, 黄飞. 可拉伸高分子光电器件的研究进展. 高分子学报, 2024, 55(9), 1091-1110

Wang, S. Y.; Zhong, W. K.; Huang, F. Recent advancements in stretchable polymer optoelectronics. Acta Polymerica Sinica, 2024, 55(9), 1091-1110
王思怡, 钟文楷, 黄飞. 可拉伸高分子光电器件的研究进展. 高分子学报, 2024, 55(9), 1091-1110 DOI： 10.11777/j.issn1000-3304.2024.24131.

Wang, S. Y.; Zhong, W. K.; Huang, F. Recent advancements in stretchable polymer optoelectronics. Acta Polymerica Sinica, 2024, 55(9), 1091-1110 DOI： 10.11777/j.issn1000-3304.2024.24131.

摘要

可拉伸高分子光电器件是一类基于共轭高分子的独特器件，具备在承受机械应变时仍能维持其光电性能的能力，在可穿戴电子、可拉伸显示、生物医学传感等领域展现出广阔的应用潜力. 近年来，国内外学者对器件与材料设计进行了大量的探索，为其性能提升和应用拓展奠定了坚实基础. 本文以外在弹性与本征弹性2个维度为切入点，深入探讨器件形态设计、材料结构调控以及薄膜组分优化等策略，总结并评述其重要成果. 最后，指出未来需要关注的重点研究方向，以克服商业化过程中面临的多重挑战，并展望可拉伸高分子器件的不断进步能为有机电子领域注入新的活力.

Abstract

Stretchable polymer optoelectronic devices

as a unique class of devices based on conjugated polymers

are capable of maintaining their optoelectronic performance under mechanical deformations. Such unique feature gives them significant potential in applications such as wearable electronics

stretchable displays

biomedical sensing and beyond. In recent years

extensive research both domestically and internationally in device and material design has laid the groundwork for enhancing the performance and expanding the applications of these devices. Currently

stretchable optoelectronic devices are primarily constructed by two approaches: external elasticity and intrinsic elasticity. Devices using external elasticity achieve stretchability through specific device forms

such as wrinkle structures

"island-bridge" structures

fiber structures

and kirigami structures. In contrast

devices based on intrinsic elasticity achieve stretchability in each functional layer through thin film modifications

such as molecular design

blending with elastomers

and adding plasticizers. This review delves into these two construction methods

examining strategies for device design

chemical modification

and thin-film composition optimization. It reviews significant research achievements in organic field-effect transistors (OFETs)

organic light-emitting diodes (OLEDs)

organic photovoltaic cells (OPVs)

and organic photodetectors (OPDs). Finally

the paper points out key research directions

highlighting challenges and opportunities in material and film modification

device engineering

and studies on structure-performance relationship. It envisions that the ongoing development of stretchable polymer optoelectronic devices will bring new vitality and breakthroughs to the field of organic electronics.

关键词

共轭聚合物可拉伸有机场效应晶体管有机发光二极管有机光探测器

Keywords

Conjugated polymersStretchableOrganic field-effect transistorsOrganic light-emitting diodesOrganic photodetectors

references

Zhu L.; Zhang M.; Xu J. Q.; Li C.; Yan J.; Zhou G. Q.; Zhong W. K.; Hao T. Y.; Song J. L.; Xue X. N.; Zhou Z. C.; Zeng R.; Zhu H. M.; Chen C. C.; MacKenzie R. C. I.; Zou Y. C.; Nelson J.; Zhang Y. M.; Sun Y. M.; Liu F. Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology. Nat. Mater., 2022, 21(6), 656-663. doi:10.1038/s41563-022-01244-yhttp://dx.doi.org/10.1038/s41563-022-01244-y

Li C.; Zhou J. D.; Song J. L.; Xu J. Q.; Zhang H. T.; Zhang X. N.; Guo J.; Zhu L.; Wei D. H.; Han G. C.; Min J.; Zhang Y.; Xie Z. Q.; Yi Y. P.; Yan H.; Gao F.; Liu F.; Sun Y. M. Non-fullerene acceptors with branched side chains and improved molecular packing to exceed 18% efficiency in organic solar cells. Nat. Energy, 2021, 6, 605-613. doi:10.1038/s41560-021-00820-xhttp://dx.doi.org/10.1038/s41560-021-00820-x

Rivnay J.; Inal S.; Salleo A.; Owens R. M.; Berggren M.; Malliaras G. G. Organic electrochemical transistors. Nat. Rev. Mater., 2018, 3(2), 17086. doi:10.1038/natrevmats.2017.86http://dx.doi.org/10.1038/natrevmats.2017.86

Kim M.; Ryu S. U.; Park S. A.; Choi K.; Kim T.; Chung D.; Park T. Donor-acceptor-conjugated polymer for high-performance organic field-effect transistors: a progress report. Adv. Funct. Mater., 2020, 30(20), 1904545. doi:10.1002/adfm.201904545http://dx.doi.org/10.1002/adfm.201904545

Zhong Z. Y.; Xu J. X.; Zhang K.; Dong M. H.; Huang Q. R.; Huang F. Unfused-ring acceptors with dithienobenzotriazole core for efficient organic solar cells. Chinese J. Polym. Sci., 2022, 40(12), 1586-1593. doi:10.1007/s10118-022-2825-yhttp://dx.doi.org/10.1007/s10118-022-2825-y

Tan X. X.; Li Y. L.; Yuan X. Y.; Kim S.; Zhang Y.; Yang C.; Huang F.; Cao Y.; Duan C. H. Polythiophene solar cells processed from non-halogenated solvent with 15.68% efficiency. Sci. China Chem., 2023, 66(8), 2347-2353. doi:10.1007/s11426-023-1695-xhttp://dx.doi.org/10.1007/s11426-023-1695-x

Tian L.; Liu C. C.; Huang F. Recent progress in side chain engineering of Y-series non-fullerene molecule and polymer acceptors. Sci. China Chem., 2024, 67(3), 788-805. doi:10.1007/s11426-023-1774-6http://dx.doi.org/10.1007/s11426-023-1774-6

Gunturkun D.; Isci R.; Faraji S.; Sütay B.; Majewski L. A.; Ozturk T. Synthesis and characterization of naphthalenediimide-thienothiophene-conjugated polymers for OFET and OPT applications. J. Mater. Chem. C, 2023, 11(38), 13129-13141. doi:10.1039/d3tc02109bhttp://dx.doi.org/10.1039/d3tc02109b

Zhong Z. M.; Peng F.; Ying L.; Huang Z. Q.; Zhong W. K.; Yu G.; Cao Y.; Huang F. Infrared photodetectors and image arrays made with organic semiconductors. Chinese J. Polym. Sci., 2023, 41(10), 1629-1637. doi:10.1007/s10118-023-2973-8http://dx.doi.org/10.1007/s10118-023-2973-8

解博名, 张凯, 李静雯, 李力, 宋煜, 崔楠, 白原青, 黄飞. 高分子学报, 2022, 53, 414-423. doi:10.11777/j.issn1000-3304.2021.21339http://dx.doi.org/10.11777/j.issn1000-3304.2021.21339

邱红, 钟知鸣, 李美静, 应磊, 俞钢, 黄飞, 曹镛. 高分子学报, 2022, 53, 433-439. doi:10.11777/j.issn1000-3304.2021.21350http://dx.doi.org/10.11777/j.issn1000-3304.2021.21350

Park J. S.; Kim G. U.; Lee S.; Lee J. W.; Li S.; Lee J. Y.; Kim B. J. Material design and device fabrication strategies for stretchable organic solar cells. Adv. Mater., 2022, 34(31), e2201623. doi:10.1002/adma.202270230http://dx.doi.org/10.1002/adma.202270230

Qin J. Q.; Lan L. K.; Chen S. S.; Huang F. N.; Shi H. R.; Chen W. J.; Xia H. B.; Sun K.; Yang C. Recent progress in flexible and stretchable organic solar cells. Adv. Funct. Mater., 2020, 30(36), 2002529. doi:10.1002/adfm.202002529http://dx.doi.org/10.1002/adfm.202002529

Dauzon E.; Sallenave X.; Plesse C.; Goubard F.; Amassian A.; Anthopoulos T. D. Pushing the limits of flexibility and stretchability of solar cells: a review. Adv. Mater., 2021, 33(36), e2101469. doi:10.1002/adma.202101469http://dx.doi.org/10.1002/adma.202101469

Park H.; Kim D. C. Structural and material-based approaches for the fabrication of stretchable light-emitting diodes. Micromachines, 2023, 15(1), 66. doi:10.3390/mi15010066http://dx.doi.org/10.3390/mi15010066

Wu F. M.; Liu Y. X.; Zhang J.; Duan S. M.; Ji D. Y.; Yang H. Recent advances in high-mobility and high-stretchability organic field-effect transistors: from materials, devices to applications. Small Methods, 2021, 5(12), e2100676. doi:10.1002/smtd.202100676http://dx.doi.org/10.1002/smtd.202100676

Chang S. H.; Koo J. H.; Yoo J.; Kim M. S.; Choi M. K.; Kim D. H.; Song Y. M. Flexible and stretchable light-emitting diodes and photodetectors for human-centric optoelectronics. Chem. Rev., 2024, 124(3), 768-859. doi:10.1021/acs.chemrev.3c00548http://dx.doi.org/10.1021/acs.chemrev.3c00548

Liu K.; Ouyang B.; Guo X. J.; Guo Y. L.; Liu Y. Q. Advances in flexible organic field-effect transistors and their applications for flexible electronics. NPJ Flex. Electron., 2022, 6, 1. doi:10.1038/s41528-022-00133-3http://dx.doi.org/10.1038/s41528-022-00133-3

Qian Y.; Zhang X. W.; Xie L. H.; Qi D. P.; Chandran B. K.; Chen X. D.; Huang W. Stretchable organic semiconductor devices. Adv. Mater., 2016, 28(42), 9243-9265. doi:10.1002/adma.201601278http://dx.doi.org/10.1002/adma.201601278

Zhang Z. T. Light-emitting materials for wearable electronics. Nat. Rev. Mater., 2022, 7, 839-840. doi:10.1038/s41578-022-00502-4http://dx.doi.org/10.1038/s41578-022-00502-4

Shi W.; Guo Y. L.; Liu Y. Q. When flexible organic field-effect transistors meet biomimetics: a prospective view of the internet of things. Adv. Mater., 2020, 32(15), e1901493. doi:10.1002/adma.201901493http://dx.doi.org/10.1002/adma.201901493

Rogers J. A.; Someya T.; Huang Y. G. Materials and mechanics for stretchable electronics. Science, 2010, 327(5973), 1603-1607. doi:10.1126/science.1182383http://dx.doi.org/10.1126/science.1182383

Lo L. W.; Zhao J. Y.; Wan H. C.; Wang Y.; Chakrabartty S.; Wang C. An inkjet-printed PEDOT:PSS-based stretchable conductor for wearable health monitoring device applications. ACS Appl. Mater. Interfaces, 2021, 13(18), 21693-21702. doi:10.1021/acsami.1c00537http://dx.doi.org/10.1021/acsami.1c00537

Root S. E.; Savagatrup S.; Printz A. D.; Rodriquez D.; Lipomi D. J. Mechanical properties of organic semiconductors for stretchable, highly flexible, and mechanically robust electronics. Chem. Rev., 2017, 117(9), 6467-6499. doi:10.1021/acs.chemrev.7b00003http://dx.doi.org/10.1021/acs.chemrev.7b00003

Yin H. X.; Zhu Y.; Youssef K.; Yu Z. B.; Pei Q. B. Structures and materials in stretchable electroluminescent devices. Adv. Mater., 2022, 34(22), 2106184. doi:10.1002/adma.202106184http://dx.doi.org/10.1002/adma.202106184

Zhao Z. Y.; Liu K.; Liu Y. W.; Guo Y. L.; Liu Y. Q. Intrinsically flexible displays: key materials and devices. Natl. Sci. Rev., 2022, 9(6), nwac090. doi:10.1093/nsr/nwac090http://dx.doi.org/10.1093/nsr/nwac090

Sun F. Q.; Jiang H.; Wang H. Y.; Zhong Y. H.; Xu Y. M.; Xing Y.; Yu M. H.; Feng L. W.; Tang Z.; Liu J.; Sun H. D.; Wang H. Z.; Wang G.; Zhu M. F. Soft fiber electronics based on semiconducting polymer. Chem. Rev., 2023, 123(8), 4693-4763. doi:10.1021/acs.chemrev.2c00720http://dx.doi.org/10.1021/acs.chemrev.2c00720

Yoo J.; Li S.; Kim D. H.; Yang J.; Choi M. K. Materials and design strategies for stretchable electroluminescent devices. Nanoscale Horiz., 2022, 7(8), 801-821. doi:10.1039/d2nh00158fhttp://dx.doi.org/10.1039/d2nh00158f

Xu X. Z.; Zhao Y.; Liu Y. Q. Wearable electronics based on stretchable organic semiconductors. Small, 2023, 19(20), 2206309. doi:10.1002/smll.202206309http://dx.doi.org/10.1002/smll.202206309

Lee H.; Jiang Z.; Yokota T.; Fukuda K.; Park S.; Someya T. Stretchable organic optoelectronic devices: design of materials, structures, and applications. Mater. Sci. Eng. R Rep., 2021, 146, 100631. doi:10.1016/j.mser.2021.100631http://dx.doi.org/10.1016/j.mser.2021.100631

Jiang Z.; Yu K.; Wang H. Y.; Rich S.; Yokota T.; Fukuda K.; Someya T. Ultraflexible integrated organic electronics for ultrasensitive photodetection. Adv. Mater. Technol., 2021, 6(1), 2000956. doi:10.1002/admt.202000956http://dx.doi.org/10.1002/admt.202000956

Lee J. W.; Phan T. N. L.; Oh E. S.; Lee H. G.; Kim T. S.; Kim B. J. Carboxylate-containing poly(thiophene vinylene) derivative with controlled molecular weights for high-performance intrinsically-stretchable organic solar cells. Adv. Funct. Mater., 2023, 33(50), 2305851. doi:10.1002/adfm.202305851http://dx.doi.org/10.1002/adfm.202305851

Trung T. Q.; Dang V. Q.; Lee H. B.; Kim D. I.; Moon S.; Lee N. E.; Lee H. An omnidirectionally stretchable photodetector based on organic-inorganic heterojunctions. ACS Appl. Mater. Interfaces, 2017, 9(41), 35958-35967. doi:10.1021/acsami.7b09411http://dx.doi.org/10.1021/acsami.7b09411

Khodagholy D.; Doublet T.; Quilichini P.; Gurfinkel M.; Leleux P.; Ghestem A.; Ismailova E.; Hervé T.; Sanaur S.; Bernard C.; Malliaras G. G. In vivo recordings of brain activity using organic transistors. Nat. Commun., 2013, 4, 1575. doi:10.1038/ncomms2573http://dx.doi.org/10.1038/ncomms2573

Zhang Z. T.; Guo K. P.; Li Y. M.; Li X. Y.; Guan G. Z.; Li H. P.; Luo Y. F.; Zhao F. Y.; Zhang Q.; Wei B.; Pei Q. B.; Peng H. S. A colour-tunable, weavable fibre-shaped polymer light-emitting electrochemical cell. Nat. Photonics, 2015, 9, 233-238. doi:10.1038/nphoton.2015.37http://dx.doi.org/10.1038/nphoton.2015.37

Hong J. H.; Shin J. M.; Kim G. M.; Joo H.; Park G. S.; Hwang I. B.; Kim M. W.; Park W. S.; Chu H. Y.; Kim S. 9.1-inch stretchable AMOLED display based on LTPS technology. J. Soc. Inf. Disp., 2017, 25(3), 194-199. doi:10.1002/jsid.547http://dx.doi.org/10.1002/jsid.547

Hu X. Y.; Dou Y. Y.; Li J. J.; Liu Z. F. Buckled structures: fabrication and applications in wearable electronics. Small, 2019, 15(32), e1804805. doi:10.1002/smll.201970169http://dx.doi.org/10.1002/smll.201970169

Lipomi D. J.; Tee B. C. K.; Vosgueritchian M.; Bao Z. N. Stretchable organic solar cells. Adv. Mater., 2011, 23(15), 1771-1775. doi:10.1002/adma.201004426http://dx.doi.org/10.1002/adma.201004426

White M. S.; Kaltenbrunner M.; Głowacki E. D.; Gutnichenko K.; Kettlgruber G.; Graz I.; Aazou S.; Ulbricht C.; Egbe D. A. M.; Miron M. C.; Major Z.; Scharber M. C.; Sekitani T.; Someya T.; Bauer S.; Sariciftci N. S. Ultrathin, highly flexible and stretchable PLEDs. Nat. Photonics, 2013, 7, 811-816. doi:10.1038/nphoton.2013.188http://dx.doi.org/10.1038/nphoton.2013.188

Kaltenbrunner M.; White M. S.; Głowacki E. D.; Sekitani T.; Someya T.; Sariciftci N. S.; Bauer S. Ultrathin and lightweight organic solar cells with high flexibility. Nat. Commun., 2012, 3, 770. doi:10.1038/ncomms1772http://dx.doi.org/10.1038/ncomms1772

Huang W. C.; Jiang Z.; Fukuda K.; Jiao X. C.; McNeill C. R.; Yokota T.; Someya T. Efficient and mechanically robust ultraflexible organic solar cells based on mixed acceptors. Joule, 2020, 4(1), 128-141. doi:10.1016/j.joule.2019.10.007http://dx.doi.org/10.1016/j.joule.2019.10.007

Park S.; Fukuda K.; Wang M.; Lee C.; Yokota T.; Jin H.; Jinno H.; Kimura H.; Zalar P.; Matsuhisa N.; Umezu S.; Bazan G. C.; Someya T. Ultraflexible near-infrared organic photodetectors for conformal photoplethysmogram sensors. Adv. Mater., 2018, 30, 1802359. doi:10.1002/adma.201870252http://dx.doi.org/10.1002/adma.201870252

Yin D.; Feng J.; Ma R.; Liu Y. F.; Zhang Y. L.; Zhang X. L.; Bi Y. G.; Chen Q. D.; Sun H. B. Efficient and mechanically robust stretchable organic light-emitting devices by a laser-programmable buckling process. Nat. Commun., 2016, 7, 11573. doi:10.1038/ncomms11573http://dx.doi.org/10.1038/ncomms11573

Jeong S.; Yoon H.; Lee B.; Lee S.; Hong Y. Distortion-free stretchable light-emitting diodes via imperceptible microwrinkles. Adv. Mater. Technol., 2020, 5(9), 2000231. doi:10.1002/admt.202070057http://dx.doi.org/10.1002/admt.202070057

Park T. H.; Ren W. Q.; Lee H. J.; Kim N.; Son K. R.; Rani A.; Kim T. G. Efficient TADF-based blue OLEDs with 100% stretchability using titanium particle-embedded indium zinc oxide mesh electrodes. NPG Asia Mater., 2022, 14, 66. doi:10.1038/s41427-022-00411-6http://dx.doi.org/10.1038/s41427-022-00411-6

Yao L. Q.; Qin Y.; Li X. C.; Xue Q.; Liu F.; Cheng T.; Li G. J.; Zhang X. W.; Lai W. Y. High-efficiency stretchable organic light-emitting diodes based on ultra-flexible printed embedded metal composite electrodes. InfoMat, 2023, 5(5), e12410. doi:10.1002/inf2.12410http://dx.doi.org/10.1002/inf2.12410

Sekitani T.; Noguchi Y.; Hata K. J.; Fukushima T.; Aida T.; Someya T. A rubberlike stretchable active matrix using elastic conductors. Science, 2008, 321(5895), 1468-1472. doi:10.1126/science.1160309http://dx.doi.org/10.1126/science.1160309

Cho H.; Lee B.; Jang D.; Yoon J.; Chung S.; Hong Y. Recent progress in strain-engineered elastic platforms for stretchable thin-film devices. Mater. Horiz., 2022, 9(8), 2053-2075. doi:10.1039/d2mh00470dhttp://dx.doi.org/10.1039/d2mh00470d

Lim M. S.; Nam M.; Choi S.; Jeon Y.; Son Y. H.; Lee S. M.; Choi K. C. Two-dimensionally stretchable organic light-emitting diode with elastic pillar arrays for stress relief. Nano Lett., 2020, 20(3), 1526-1535. doi:10.1021/acs.nanolett.9b03657http://dx.doi.org/10.1021/acs.nanolett.9b03657

Kim T.; Lee H.; Jo W.; Kim T. S.; Yoo S. Realizing stretchable OLEDs: a hybrid platform based on rigid island arrays on a stress-relieving bilayer structure. Adv. Mater. Technol., 2020, 5(11), 2000494. doi:10.1002/admt.202070068http://dx.doi.org/10.1002/admt.202070068

Kang I.; Yun H. J.; Chung D. S.; Kwon S. K.; Kim Y. H. Record high hole mobility in polymer semiconductors via side-chain engineering. J. Am. Chem. Soc., 2013, 135(40), 14896-14899. doi:10.1021/ja405112shttp://dx.doi.org/10.1021/ja405112s

Wang W. C.; Wang S. H.; Rastak R.; Ochiai Y.; Niu S. M.; Jiang Y. W.; Arunachala P. K.; Zheng Y.; Xu J.; Matsuhisa N.; Yan X. Z.; Kwon S. K.; Miyakawa M.; Zhang Z. T.; Ning R.; Foudeh A. M.; Yun Y.; Linder C.; Tok J. B. H.; Bao Z. N. Strain-insensitive intrinsically stretchable transistors and circuits. Nat. Electron., 2021, 4, 143-150. doi:10.1038/s41928-020-00525-1http://dx.doi.org/10.1038/s41928-020-00525-1

Su R. T.; Park S. H.; Ouyang X.; Ahn S. I.; McAlpine M. C. 3D-printed flexible organic light-emitting diode displays. Sci. Adv., 2022, 8(1), eabl8798. doi:10.1126/sciadv.abl8798http://dx.doi.org/10.1126/sciadv.abl8798

Fakharuddin A.; Li H. Z.; Di Giacomo F.; Zhang T. Y.; Gasparini N.; Elezzabi A. Y.; Mohanty A.; Ramadoss A.; Ling J.; Soultati A.; Tountas M.; Schmidt-Mende L.; Argitis P.; Jose R.; Nazeeruddin M. K.; Bin Mohd Yusoff A. R.; Vasilopoulou M. Fiber-shaped electronic devices. Adv. Energy Mater., 2021, 11(34), 2101443. doi:10.1002/aenm.202101443http://dx.doi.org/10.1002/aenm.202101443

Hamedi M.; Forchheimer R.; Inganäs O. Towards woven logic from organic electronic fibres. Nat. Mater., 2007, 6, 357-362. doi:10.1038/nmat1884http://dx.doi.org/10.1038/nmat1884

Liu J. W.; Namboothiry M. A. G.; Carroll D. L. Fiber-based architectures for organic photovoltaics. Appl. Phys. Lett., 2007, 90(6), 063501. doi:10.1063/1.2435988http://dx.doi.org/10.1063/1.2435988

Teng W. L.; Zhou Q. Q.; Wang X. K.; Che H. B.; Hu P.; Li H. Y.; Wang J. S. Hierarchically interconnected conducting polymer hybrid fiber with high specific capacitance for flexible fiber-shaped supercapacitor. Chem. Eng. J., 2020, 390, 124569. doi:10.1016/j.cej.2020.124569http://dx.doi.org/10.1016/j.cej.2020.124569

Liu P.; Gao Z.; Xu L. M.; Shi X.; Fu X. M.; Li K.; Zhang B.; Sun X. M.; Peng H. S. Polymer solar cell textiles with interlaced cathode and anode fibers. J. Mater. Chem. A, 2018, 6(41), 19947-19953. doi:10.1039/c8ta06510ahttp://dx.doi.org/10.1039/c8ta06510a

Lv D.; Jiang Q. Q.; Shang Y. Y.; Liu D. Y. Highly efficient fiber-shaped organic solar cells toward wearable flexible electronics. NPJ Flex. Electron., 2022, 6, 38. doi:10.1038/s41528-022-00172-whttp://dx.doi.org/10.1038/s41528-022-00172-w

Li H. J.; Wang W. Y.; Yang Y.; Wang Y.; Li P. F.; Huang J. H.; Li J.; Lu Y. H.; Li Z. J.; Wang Z. Z.; Fan B.; Fang J. F.; Song W. J. Kirigami-based highly stretchable thin film solar cells that are mechanically stable for more than 1000 cycles. ACS Nano, 2020, 14(2), 1560-1568. doi:10.1021/acsnano.9b06562http://dx.doi.org/10.1021/acsnano.9b06562

Zheng Y.; Zhang S.; Tok J. B. H.; Bao Z. N. Molecular design of stretchable polymer semiconductors: current progress and future directions. J. Am. Chem. Soc., 2022, 144(11), 4699-4715. doi:10.1021/jacs.2c00072http://dx.doi.org/10.1021/jacs.2c00072

Müller C.; Goffri S.; Breiby D. W.; Andreasen J. W.; Chanzy H. D.; Janssen R. A. J.; Nielsen M. M.; Radano C. P.; Sirringhaus H.; Smith P.; Stingelin‐Stutzmann N. Tough, semiconducting polyethylene-poly(3-hexylthiophene) diblock copolymers. Adv. Funct. Mater., 2007, 17(15), 2674-2679. doi:10.1002/adfm.200601248http://dx.doi.org/10.1002/adfm.200601248

Mun J.; Wang G., J N.; Oh J. Y.; Katsumata T.; Lee F. L.; Kang J.; Wu H. C.; Lissel F.; Rondeau-Gagné S.; Tok J. B. H.; Bao Z. N. Effect of nonconjugated spacers on mechanical properties of semiconducting polymers for stretchable transistors. Adv. Funct. Mater., 2018, 28(43), 1804222. doi:10.1002/adfm.201804222http://dx.doi.org/10.1002/adfm.201804222

Liu W.; Zhang C.; Alessandri R.; Diroll B. T.; Li Y.; Liang H. Y.; Fan X. C.; Wang K.; Cho H.; Liu Y. D.; Dai Y. H.; Su Q.; Li N.; Li S. S.; Wai S.; Li Q.; Shao S. Y.; Wang L. X.; Xu J.; Zhang X. H.; Talapin D. V.; de Pablo J. J.; Wang S. H. High-efficiency stretchable light-emitting polymers from thermally activated delayed fluorescence. Nat. Mater., 2023, 22(6), 737-745. doi:10.1038/s41563-023-01529-whttp://dx.doi.org/10.1038/s41563-023-01529-w

Luo X. A.; Freychet G.; Gan Z. Q.; An K.; Du H. J.; Wang C.; Li N.; Zhong W. K.; Ying L. Intrinsically stretchable organic photovoltaic thin films enabled by optimized donor-acceptor pairing. Macromolecules, 2023, 56(21), 8928-8938. doi:10.1021/acs.macromol.3c01349http://dx.doi.org/10.1021/acs.macromol.3c01349

Koch F. P. V.; Rivnay J.; Foster S.; Müller C.; Downing J. M.; Buchaca-Domingo E.; Westacott P.; Yu L. Y.; Yuan M. J.; Baklar M.; Fei Z. P.; Luscombe C.; McLachlan M. A.; Heeney M.; Rumbles G.; Silva C.; Salleo A.; Nelson J.; Smith P.; Stingelin N. The impact of molecular weight on microstructure and charge transport in semicrystalline polymer semiconductors-poly(3-hexylthiophene), studyamodel. Prog. Polym. Sci., 2013, 38(12), 1978-1989. doi:10.1016/j.progpolymsci.2013.07.009http://dx.doi.org/10.1016/j.progpolymsci.2013.07.009

Lee J. W.; Kim G. U.; Kim D. J.; Jeon Y.; Li S.; Kim T. S.; Lee J. Y.; Kim B. J. Intrinsically-stretchable, efficient organic solar cells achieved by high-molecular-weight, electro-active polymer acceptor additives. Adv. Energy Mater., 2022, 12(28), 2200887. doi:10.1002/aenm.202200887http://dx.doi.org/10.1002/aenm.202200887

Zhu Q. L.; Xue J. W.; Zhang L.; Wen J. L.; Lin B. J.; Naveed H. B.; Bi Z. Z.; Xin J. M.; Zhao H.; Zhao C.; Zhou K.; Liu S. F.; Ma W. Intermolecular interaction control enables co-optimization of efficiency, deformability, mechanical and thermal stability of stretchable organic solar cells. Small, 2021, 17(21), e2007011. doi:10.1002/smll.202170100http://dx.doi.org/10.1002/smll.202170100

Song W.; Yu K. B.; Ge J. F.; Xie L.; Zhou R.; Peng R. X.; Zhang X. L.; Yang M. J.; Wei Z. X.; Ge Z. Y. Entangled structure morphology by polymer guest enabling mechanically robust organic solar cells with efficiencies of over 16.5%. Matter, 2022, 5(6), 1877-1889. doi:10.1016/j.matt.2022.03.012http://dx.doi.org/10.1016/j.matt.2022.03.012

Wang Z. Y.; Zhang D.; Xu M. C.; Liu J. F.; He J. Y.; Yang L. P.; Li Z. L.; Gao Y. R.; Shao M. Intrinsically stretchable organic solar cells with simultaneously improved mechanical robustness and morphological stability enabled by a universal crosslinking strategy. Small, 2022, 18(26), e2201589. doi:10.1002/smll.202201589http://dx.doi.org/10.1002/smll.202201589

Oh J. Y.; Rondeau-Gagné S.; Chiu Y. C.; Chortos A.; Lissel F.; Wang G.J N.; Schroeder B. C.; Kurosawa T.; Lopez J.; Katsumata T.; Xu J.; Zhu C. X.; Gu X. D.; Bae W. G.; Kim Y.; Jin L. H.; Chung J. W.; Tok J. B. H.; Bao Z. N.Intrinsically stretchable and healable semiconducting polymer for organic transistors. Nature, 2016, 539(7629), 411-415. doi:10.1038/nature20102http://dx.doi.org/10.1038/nature20102

Lee J. W.; Seo S.; Lee S. W.; Kim G. U.; Han S.; Phan T. N. L.; Lee S.; Li S.; Kim T. S.; Lee J. Y.; Kim B. J. Intrinsically stretchable, highly efficient organic solar cells enabled by polymer donors featuring hydrogen-bonding spacers. Adv. Mater., 2022, 34(50), e2207544. doi:10.1002/adma.202270344http://dx.doi.org/10.1002/adma.202270344

Noh J.; Kim G. U.; Han S.; Oh S. J.; Jeon Y.; Jeong D.; Kim S. W.; Kim T. S.; Kim B. J.; Lee J. Y. Intrinsically stretchable organic solar cells with efficiencies of over 11%. ACS Energy Lett., 2021, 6(7), 2512-2518. doi:10.1021/acsenergylett.1c00829http://dx.doi.org/10.1021/acsenergylett.1c00829

Son S. Y.; Kim J. H.; Song E.; Choi K.; Lee J.; Cho K.; Kim T. S.; Park T. Exploiting π-π stacking for stretchable semiconducting polymers. Macromolecules, 2018, 51(7), 2572-2579. doi:10.1021/acs.macromol.8b00093http://dx.doi.org/10.1021/acs.macromol.8b00093

Li M. F.; Xian K. H.; Zhao W. C.; Sheng D.; Liu C. H.; Li X.; Li W. W.; Ye L. Optimizing mechanical stretchability and photovoltaic performance in all-polymer solar cells from a two-donor polymer blend. Chem. Eng. J., 2023, 476, 146723. doi:10.1016/j.cej.2023.146723http://dx.doi.org/10.1016/j.cej.2023.146723

Wan Q. P.; Seo S.; Lee S. W.; Lee J.; Jeon H.; Kim T. S.; Kim B. J.; Thompson B. C. High-performance intrinsically stretchable polymer solar cell with record efficiency and stretchability enabled by thymine-functionalized terpolymer. J. Am. Chem. Soc., 2023, 145(22), 11914-11920. doi:10.1021/jacs.3c02764http://dx.doi.org/10.1021/jacs.3c02764

Choi D.; Kim H.; Persson N.; Chu P. H.; Chang M.; Kang J. H.; Graham S.; Reichmanis E. Elastomer-polymer semiconductor blends for high-performance stretchable charge transport networks. Chem. Mater., 2016, 28(4), 1196-1204. doi:10.1021/acs.chemmater.5b04804http://dx.doi.org/10.1021/acs.chemmater.5b04804

Jeon K. H.; Park J. W. Light-emitting polymer blended with elastomers for stretchable polymer light-emitting diodes. Macromolecules, 2022, 55(18), 8311-8320. doi:10.1021/acs.macromol.2c01095http://dx.doi.org/10.1021/acs.macromol.2c01095

Park Y.; Fuentes-Hernandez C.; Kim K.; Chou W. F.; Larrain F. A.; Graham S.; Pierron O. N.; Kippelen B. Skin-like low-noise elastomeric organic photodiodes. Sci. Adv., 2021, 7(51), eabj6565. doi:10.1126/sciadv.abj6565http://dx.doi.org/10.1126/sciadv.abj6565

Peng Z. X.; Xian K. H.; Cui Y.; Qi Q. C.; Liu J. W.; Xu Y.; Chai Y. B.; Yang C. M.; Hou J. H.; Geng Y. H.; Ye L. Thermoplastic elastomer tunes phase structure and promotes stretchability of high-efficiency organic solar cells. Adv. Mater., 2021, 33(49), e2106732. doi:10.1002/adma.202106732http://dx.doi.org/10.1002/adma.202106732

Yu Z. B.; Niu X. F.; Liu Z. T.; Pei Q. B. Intrinsically stretchable polymer light-emitting devices using carbon nanotube-polymer composite electrodes. Adv. Mater., 2011, 23(34), 3989-3994. doi:10.1002/adma.201101986http://dx.doi.org/10.1002/adma.201101986

Xu J.; Wang S. H.; Wang G.J N.; Zhu C. X.; Luo S. C.; Jin L. H.; Gu X. D.; Chen S. C.; Feig V. R.; To J. W. F.; Rondeau-Gagné S.; Park J.; Schroeder B. C.; Lu C. E.; Oh J. Y.; Wang Y. M.; Kim Y. H.; Yan H.; Sinclair R.; Zhou D. S.; Xue G.; Murmann B.; Linder C.; Cai W.; Tok J. B. H.; Chung J. W.; Bao Z. N.Highly stretchable polymer semiconductor films through the nanoconfinement effect. Science, 2017, 355(6320), 59-64. doi:10.1126/science.aah4496http://dx.doi.org/10.1126/science.aah4496

Xu J.; Wu H. C.; Zhu C. X.; Ehrlich A.; Shaw L.; Nikolka M.; Wang S. H.; Molina-Lopez F.; Gu X. D.; Luo S. C.; Zhou D. S.; Kim Y. H.; Wang G.J N.; Gu K.; Feig V. R.; Chen S. C.; Kim Y.; Katsumata T.; Zheng Y. Q.; Yan H.; Chung J. W.; Lopez J.; Murmann B.; Bao Z. N. Multi-scale ordering in highly stretchable polymer semiconducting films. Nat. Mater., 2019, 18(6), 594-601. doi:10.1038/s41563-019-0340-5http://dx.doi.org/10.1038/s41563-019-0340-5

Zhang Z.; Wang W.; Jiang Y.; Wang Y. X.; Wu Y.; Lai J. C.; Niu S.; Xu C.; Shih C. C.; Wang C.; Yan H.; Galuska L.; Prine N.; Wu H. C.; Zhong D.; Chen G.; Matsuhisa N.; Zheng Y.; Yu Z.; Wang Y.; Dauskardt R.; Gu X.; Tok J. B.; Bao Z. High-brightness all-polymer stretchable LED with charge-trapping dilution. Nature, 2022, 603(7902), 624-630. doi:10.1038/s41586-022-04400-1http://dx.doi.org/10.1038/s41586-022-04400-1

Jeong M. W.; Ma J. H.; Shin J. S.; Kim J. S.; Ma G. R.; Nam T. U.; Gu X. D.; Kang S. J.; Oh J. Y. Intrinsically stretchable three primary light-emitting films enabled by elastomer blend for polymer light-emitting diodes. Sci. Adv., 2023, 9(25), eadh1504. doi:10.1126/sciadv.adh1504http://dx.doi.org/10.1126/sciadv.adh1504

Li S. M.; Gao M. Y.; Zhou K. K.; Li X.; Xian K. H.; Zhao W. C.; Chen Y.; He C. Y.; Ye L. Achieving record-high stretchability and mechanical stability in organic photovoltaic blends with a dilute-absorber strategy. Adv. Mater., 2024, 36(8), 2307278. doi:10.1002/adma.202307278http://dx.doi.org/10.1002/adma.202307278

Zheng X. J.; Wu X. L.; Wu Q.; Han Y. F.; Ding G. Y.; Wang Y. M.; Kong Y. B.; Chen T. Y.; Wang M. T.; Zhang Y. Q.; Xue J. W.; Fu W. F.; Luo Q.; Ma C. Q.; Ma W.; Zuo L. J.; Shi M. M.; Chen H. Z. Thorough optimization for intrinsically stretchable organic photovoltaics. Adv. Mater., 2024, 36(11), e2307280. doi:10.1002/adma.202307280http://dx.doi.org/10.1002/adma.202307280

Han J. H.; Bao F.; Huang D.; Wang X. C.; Yang C. M.; Yang R. Q.; Jian X. G.; Wang J. Y.; Bao X. C.; Chu J. H. A universal method to enhance flexibility and stability of organic solar cells by constructing insulating matrices in active layers. Adv. Funct. Mater., 2020, 30(38), 2003654. doi:10.1002/adfm.202003654http://dx.doi.org/10.1002/adfm.202003654

Liu Y. W.; Zhu M. L.; Sun J. Z.; Shi W. K.; Zhao Z. Y.; Wei X. F.; Huang X.; Guo Y. L.; Liu Y. Q. A self-assembled 3D penetrating nanonetwork for high-performance intrinsically stretchable polymer light-emitting diodes. Adv. Mater., 2022, 34(27), e2201844. doi:10.1002/adma.202201844http://dx.doi.org/10.1002/adma.202201844

Paleti S. H. K.; Kim Y.; Kimpel J.; Craighero M.; Haraguchi S.; Müller C. Impact of doping on the mechanical properties of conjugated polymers. Chem. Soc. Rev., 2024, 53(4), 1702-1729. doi:10.1039/d3cs00833ahttp://dx.doi.org/10.1039/d3cs00833a

Kim J. H.; Park J. W. Intrinsically stretchable organic light-emitting diodes. Sci. Adv., 2021, 7(9), eabd9715. doi:10.1126/sciadv.abd9715http://dx.doi.org/10.1126/sciadv.abd9715

Zhuo Z. Q.; Ni M. J.; An X.; Bai L. B.; Liang X. Y.; Yang J.; Zheng Y. Y.; Liu B.; Sun N.; Sun L. L.; Wei C. X.; Yu N. N.; Chen W. Y.; Li M. Y.; Xu M.; Lin J. Y.; Huang W. Intrinsically stretchable and efficient fully π-conjugated polymer via internal plasticization for flexible deep-blue polymer light-emitting diodes with CIEy = 0.08. Adv. Mater., 2023, 35(40), 2303923. doi:10.1002/adma.202303923http://dx.doi.org/10.1002/adma.202303923

Wang Z. Y.; Xu M. C.; Li Z. L.; Gao Y. R.; Yang L. P.; Zhang D.; Shao M. Intrinsically stretchable organic solar cells beyond 10% power conversion efficiency enabled by transfer printing method. Adv. Funct. Mater., 2021, 31(35), 2103534. doi:10.1002/adfm.202103534http://dx.doi.org/10.1002/adfm.202103534

Fan X.; Nie W. Y.; Tsai H.; Wang N. X.; Huang H. H.; Cheng Y. J.; Wen R. J.; Ma L. J.; Yan F.; Xia Y. G. PEDOT:PSS for flexible and stretchable electronics: modifications, strategies, and applications. Adv. Sci., 2019, 6(19), 1900813. doi:10.1002/advs.201900813http://dx.doi.org/10.1002/advs.201900813

Kayser L. V.; Lipomi D. J. Stretchable conductive polymers and composites based on PEDOT and PEDOT:PSS. Adv. Mater., 2019, 31(10), e1806133. doi:10.1002/adma.201806133http://dx.doi.org/10.1002/adma.201806133

Vosgueritchian M.; Lipomi D. J.; Bao Z. N. Highly conductive and transparent PEDOT:PSS films with a fluorosurfactant for stretchable and flexible transparent electrodes. Adv. Funct. Mater., 2012, 22(2), 421-428. doi:10.1002/adfm.201101775http://dx.doi.org/10.1002/adfm.201101775

Kim J. Y.; Jung J. H.; Lee D. E.; Joo J. Enhancement of electrical conductivity of poly(3,4-ethylenedioxythiophene)/poly(4-styrenesulfonate) by a change of solvents. Synth. Met., 2002, 126(2-3), 311-316. doi:10.1016/s0379-6779(01)00576-8http://dx.doi.org/10.1016/s0379-6779(01)00576-8

Wang Y.; Zhu C. X.; Pfattner R.; Yan H. P.; Jin L. H.; Chen S. C.; Molina-Lopez F.; Lissel F.; Liu J.; Rabiah N. I.; Chen Z.; Chung J. W.; Linder C.; Toney M. F.; Murmann B.; Bao Z. N. A highly stretchable, transparent, and conductive polymer. Sci. Adv., 2017, 3(3), e1602076. doi:10.1126/sciadv.1602076http://dx.doi.org/10.1126/sciadv.1602076

Shin E. Y.; Park S. H.; Jeon Y.; Kim K.; Lee G.; Lee J. Y.; Son H. J. Important role of additive in morphology of stretchable electrode for highly intrinsically stable organic photovoltaics. ACS Appl. Energy Mater., 2023, 6(17), 8729-8737. doi:10.1021/acsaem.3c01204http://dx.doi.org/10.1021/acsaem.3c01204

Wang X. M.; Liu Y. Q.; Chen Q. Z.; Yan Y. J.; Rao Z. C.; Lin Z. X.; Chen H. P.; Guo T. L. Recent advances in stretchable field-effect transistors. J. Mater. Chem. C, 2021, 9(25), 7796-7828. doi:10.1039/d1tc01082dhttp://dx.doi.org/10.1039/d1tc01082d

Cui N.; Song Y.; Tan C. H.; Zhang K.; Yang X. Y.; Dong S.; Xie B. M.; Huang F. Stretchable transparent electrodes for conformable wearable organic photovoltaic devices. NPJ Flex. Electron., 2021, 5, 31. doi:10.1038/s41528-021-00127-7http://dx.doi.org/10.1038/s41528-021-00127-7

Chen Z. H.; Fang R.; Li W.; Guan J. G. Stretchable transparent conductors: from micro/macromechanics to applications. Adv. Mater., 2019, 31(35), e1900756. doi:10.1002/adma.201900756http://dx.doi.org/10.1002/adma.201900756

Oyewole O.; Oyewole D.; Oyelade O.; Adeniji S.; Koech R.; Asare J.; Agyei-Tuffour B.; Soboyejo W. Failure of stretchable organic solar cells under monotonic and cyclic loading. Macromol. Mater. Eng., 2020, 305(11), 2000369. doi:10.1002/mame.202000369http://dx.doi.org/10.1002/mame.202000369

Steinmann V.; Moro L. Encapsulation requirements to enable stable organic ultra-thin and stretchable devices. J. Mater. Res., 2018, 33(13), 1925-1936. doi:10.1557/jmr.2018.194http://dx.doi.org/10.1557/jmr.2018.194

Liang J. J.; Li L.; Chen D.; Hajagos T.; Ren Z.; Chou S. Y.; Hu W.; Pei Q. B. Intrinsically stretchable and transparent thin-film transistors based on printable silver nanowires, carbon nanotubes and an elastomeric dielectric. Nat. Commun., 2015, 6, 7647. doi:10.1038/ncomms8647http://dx.doi.org/10.1038/ncomms8647

Liu J.; Wang J. C.; Zhang Z. T.; Molina-Lopez F.; Wang G.J N.; Schroeder B. C.; Yan X. Z.; Zeng Y. T.; Zhao O.; Tran H.; Lei T.; Lu Y.; Wang Y. X.; Tok J. B. H.; Dauskardt R.; Chung J. W.; Yun Y.; Bao Z. N.Fully stretchable active-matrix organic light-emitting electrochemical cell array. Nat. Commun., 2020, 11(1), 3362. doi:10.1038/s41467-020-17084-whttp://dx.doi.org/10.1038/s41467-020-17084-w

Yin D.; Jiang N. R.; Chen Z. Y.; Liu Y. F.; Bi Y. G.; Zhang X. L.; Feng J.; Sun H. B. Roller-assisted adhesion imprinting for high-throughput manufacturing of wearable and stretchable organic light-emitting devices. Adv. Opt. Mater., 2020, 8(4), 1901525. doi:10.1002/adom.201901525http://dx.doi.org/10.1002/adom.201901525

Zhang S.; Alesadi A.; Mason G. T.; Chen K. L.; Freychet G.; Galuska L.; Cheng Y. H.; St Onge P. B. J.; Ocheje M. U.; Ma G. R.; Qian Z. Y.; Dhakal S.; Ahmad Z.; Wang C.; Chiu Y. C.; Rondeau-Gagné S.; Xia W. J.; Gu X. D. Molecular origin of strain-induced chain alignment in PDPP-based semiconducting polymeric thin films. Adv. Funct. Mater., 2021, 31(21), 2100161. doi:10.1002/adfm.202100161http://dx.doi.org/10.1002/adfm.202100161

Gao Y. R.; Liao J. W.; Chen H. Y.; Ning H. J.; Wu Q. H.; Li Z. L.; Wang Z. Y.; Zhang X. L.; Shao M.; Yu Y. High performance polarization-resolved photodetectors based on intrinsically stretchable organic semiconductors. Adv. Sci., 2023, 10(2), e2204727. doi:10.1002/advs.202204727http://dx.doi.org/10.1002/advs.202204727

Sen P.; Yang R. N.; Rech J. J.; Feng Y. X.; Ho C. H. Y.; Huang J. S.; So F.; Kline R. J.; You W.; Kudenov M. W.; O'Connor B. T. Panchromatic all-polymer photodetector with tunable polarization sensitivity. Adv. Opt. Mater., 2019, 7(4), 1801346. doi:10.1002/adom.201801346http://dx.doi.org/10.1002/adom.201801346

Views

395

下载量

CSCD

Alert me when the article has been cited

提交

Tools

Publicity Resources

Synthesis and Semiconducting Properties of Conjugated Polymers Based on Fluorinated Isoindigo[7, 6-g]isoindigo

Design, Synthesis and Properties of Self-healing Luminescent Elastomers with Hydrogen-bonded Side-chain-modified Conjugated Polymer Backbones

Recent Progress of Conjugated Polymers Containing Quinoidal Structure

A Near-infrared Electron Acceptor with Thieno[3,4-b]thiophene as the Core and the Related High-performance Photodetectors

Related Author

Yu Jiang

Yao Gao

Hong-kun Tian

Jun-qiao Ding

Yan-hou Geng

Fo-song Wang

Yi Wan

Xiang-chun Li

Related Institution

University of Chinese Academy of Sciences

School of Material Science and Engineering, Collaborative Innovation Center of Chemical Science and Engineering(Tianjin), Tianjin University

State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences

State Key Laboratory of Organic Electronics and Information Displays, School of Chemistry and Life Sciences, Nanjing University of Posts & Telecommunications

School of Materials Science and Engineering, Tianjin University

Postal code：100190
Tel：010-62588927 Email：gfzxb@iccas.ac.cn
Technical support is provided by Beijing Founder electronics co., LTD 京ICP备05002797号-8 京公网安备11010802024621
It is recommended to read the content of this site in Chrome&IE9+. Please switch to extreme mode in browser 360.
Cookies We use cookies to help provide and enhance our service and tailor content. By continuing, you agree to the use of cookies.

⁰