Structure and Property Regulation of Polymer Semiconductors <italic style="font-style: italic">via</italic> Epitaxial Crystallization

Jing-yue Yan; Yu-min Liu; Hua-dong Huang; Can Gao; Huan-li Dong; Zhong-ming Li

doi:10.11777/j.issn1000-3304.2024.24152

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Structure and Property Regulation of Polymer Semiconductors via Epitaxial Crystallization

Review | 更新时间：2024-12-24

- Structure and Property Regulation of Polymer Semiconductors via Epitaxial Crystallization
- Acta Polymerica Sinica Vol. 55, Issue 11, Pages: 1441-1462(2024)
- 作者机构：
  
  1.中国科学院化学研究所北京分子科学国家重点实验室北京 100190
  2.四川大学高分子科学与工程学院四川 610065
  3.中国科学院大学北京 100049
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2024.24152
  CLC：
- CSTR：32057.14.GFZXB.2024.7267
- Received：27 May 2024，
  
  Accepted：2024-06-28，
  
  Published Online：24 September 2024，
  
  Published：20 November 2024
- 稿件说明：
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闫敬越, 刘玉敏, 黄华东, 高灿, 董焕丽, 李忠明. 附生结晶调控有机高分子半导体材料聚集态结构与性能. 高分子学报, 2024, 55(11), 1441-1462

Yan, J. Y.; Liu, Y. M.; Huang, H. D.; Gao, C; Dong, H. L.; Li, Z. M. Structure and property regulation of polymer semiconductors via epitaxial crystallization. Acta Polymerica Sinica, 2024, 55(11), 1441-1462
闫敬越, 刘玉敏, 黄华东, 高灿, 董焕丽, 李忠明. 附生结晶调控有机高分子半导体材料聚集态结构与性能. 高分子学报, 2024, 55(11), 1441-1462 DOI： 10.11777/j.issn1000-3304.2024.24152. CSTR： 32057.14.GFZXB.2024.7267.

Yan, J. Y.; Liu, Y. M.; Huang, H. D.; Gao, C; Dong, H. L.; Li, Z. M. Structure and property regulation of polymer semiconductors via epitaxial crystallization. Acta Polymerica Sinica, 2024, 55(11), 1441-1462 DOI： 10.11777/j.issn1000-3304.2024.24152. CSTR： 32057.14.GFZXB.2024.7267.

摘要

高质量共轭高分子半导体晶体材料的制备对于其基础物性的研究和高性能有机光电器件的构筑具有至关重要的意义. 但是高分子材料存在本征分子量大、呈分散性、链间易于缠结等特征，导致其高度有序共轭高分子聚集体的制备面临巨大挑战. 本文立足于有机高分子半导体材料聚集态结构与性能调控，在传统溶液组装策略的基础上，介绍了新型取向结晶策略，重点探讨了附生结晶的影响因素以及附生结晶在调控有机高分子半导体材料聚集态结构与性能方面的优势，并对目前附生结晶存在的问题进行了总结与展望.

Abstract

The field of organic electronics has made significant progress after more than 40 years of research

giving rise to a series of emerging related areas. Due to limitations such as limited conjugated size of small molecules and high degree of disorders in conjugated polymers

research in this field is currently facing performance limits and its development is distinctly hindered. The preparation of high-quality semiconductor crystals of conjugated polymers is of great significance for the study of their basic physical properties and the construction of organic optoelectronic devices with the high performance. However

due to the inherent characteristics such as high molecular weight

dispersibility

and easy entanglement between chains

the acquisition of highly ordered aggregates for conjugated polymers faces enormous challenges. Study on the crystallization of conjugated polymers is definitely important for preparing their high-quality crystals in order to overcome the current performance limitations in organic electronics

and would be expected to provide an important research platform for basic physical properties of conjugated polymers. Epitaxial crystallization is a surface-induced crystallization method. The existence of oriented substrate can reduce the nucleation barrier of crystallization processes and make the crystallization processes more easily to occur in comparison to the traditional solution crystallization. Therefore

epitaxial crystallization has become a common method for regulating the aggregation structure and properties of organic polymer semiconductor materials. In this contribution

we first briefly introduced the regulation of the aggregate structures of organic polymer semiconductor materials through traditional solution assembly and new oriented crystallization strategies. The factors of epitaxial crystallization and their advantages on regulating the aggregate structures and properties of organic polymer semiconductor materials were then particularly summarized. Future study on epitaxial crystallization in organic conjugated polymers was prospected in the end.

关键词

Keywords

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Related Author

Du-jin Wang

Xia Dong

Ping Zhu

Li-li Wang

De-hua Xin

Rong Hu

An-jun Qin

Ben Zhong Tang

Related Institution

Beijing National Laboratory for Molecular Science, CAS Key Laboratory of Engineering Plastics, Institute of Chemistry, Chinese Academy of Sciences

State Key Laboratory of Bio-Fibers and Eco-Textiles, Institute of Marine Biobased Materials, Qingdao University

State Key Laboratory of Luminescent Materials and Devices, South China University of Technology

Department of Chemistry, Hong Kong Branch of Chinese National Engineering Research Center for Tissue Resto-ration and Reconstruction, The Hong Kong University of Science & Technology

State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences

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Structure and Property Regulation of Polymer Semiconductors via Epitaxial Crystallization

DOI：10.11777/j.issn1000-3304.2024.24152

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Abstract

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