The Core-shell Structure and Functionality of Carbonized Polymer Dots

Da Yue; Tang-lue Feng; Bai Yang

doi:10.11777/j.issn1000-3304.2021.21105

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The Core-shell Structure and Functionality of Carbonized Polymer Dots

Reviews | 更新时间：2022-09-30

- The Core-shell Structure and Functionality of Carbonized Polymer Dots
- ACTA POLYMERICA SINICA Vol. 52, Issue 8, Pages: 938-959(2021)
- 作者机构：
  
  超分子结构与材料国家重点实验室吉林大学化学学院长春 130012
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2021.21105
  CLC：
- Published：20 August 2021，
  
  Published Online：01 July 2021，
  
  Received：09 April 2021，
  
  Revised：30 April 2021，
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乐妲,冯唐略,杨柏.碳化聚合物点的核壳结构与功能[J].高分子学报,2021,52(08):938-959.

Yue Da,Feng Tang-lue,Yang Bai.The Core-shell Structure and Functionality of Carbonized Polymer Dots[J].ACTA POLYMERICA SINICA,2021,52(08):938-959.
乐妲,冯唐略,杨柏.碳化聚合物点的核壳结构与功能[J].高分子学报,2021,52(08):938-959. DOI： 10.11777/j.issn1000-3304.2021.21105.

Yue Da,Feng Tang-lue,Yang Bai.The Core-shell Structure and Functionality of Carbonized Polymer Dots[J].ACTA POLYMERICA SINICA,2021,52(08):938-959. DOI： 10.11777/j.issn1000-3304.2021.21105.

摘要

碳化聚合物点作为一类新型的荧光碳纳米点，其高量子产率、独特的碳核和聚合物壳的杂化结构和功能在近些年引起了广泛关注. 本文通过系统总结、分析相关文献，揭示了碳化聚合物点不仅具有碳点的典型性质，也具有聚合物的性质. 强调了碳化聚合物点的聚合-碳化的本质，并详细讨论了碳化聚合物点的结构特点、制备方法方面的普适性和规律性以及光致发光的机制. 最后，基于碳化聚合物点的结构和性能调控，综述了其在传感、光电器件、催化和生物医学等不同领域的应用，并对碳化聚合物点的发展前景进行了展望.

Abstract

As a new type of fluorescent carbon nanodots

carbonized polymer dots (CPDs) have attracted extensive attention in recent years due to their unique hybrid structure and functionalities of carbon core and polymer shell. This review systematically summarizes and analyzes the relevant literature

and reveals that CPDs have the properties of both traditional carbon dots and polymers. CPDs

showing aggregated/crosslinked and carbonized polymer hybrid nanostructures

are often produced from small molecules

polymers

or biomass by assembling

polymerization

crosslinking

and carbonization

via

"bottom-up" methods. We emphasize the important role of polymerization and carbonization during the formation of CPDs

which is the essence of the CPDs. Due to the abundance of carbon sources and various synthetic strategies

the structure and properties of CPDs are diverse. Moreover

we discuss the photoluminescence mechanism of CPDs

and systematically conclude that the complicated influence factors of photoluminescence can be mainly classified as molecule state

carbon core state

surface state and crosslink enhanced emission (CEE) effect. CPDs are endowed with many unique optical

electrical and other physical and chemical properties

which are attributed to the polymer/carbon hybrid structure. Finally

based on the structure and performance control on CPDs

the applications of CPDs in different fields such as sensing

optoelectronic devices

catalysis and biomedicine are reviewed

and the development prospect of CPDs is discussed.

关键词

碳化聚合物点碳点发光机理碳核聚合物壳

Keywords

Carbonized polymer dotsCarbon dotsPhotoluminescence mechanismCarbon corePolymer shell

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