Application of Polymerization-induced Self-assembly (PISA) Technology

Bo-yang Shi; Guo-wei Wang

doi:10.11777/j.issn1000-3304.2021.21156

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Application of Polymerization-induced Self-assembly (PISA) Technology

Review | 更新时间：2024-10-08

- Application of Polymerization-induced Self-assembly (PISA) Technology
- ACTA POLYMERICA SINICA Vol. 53, Issue 1, Pages: 15-29(2022)
- 作者机构：
  
  复旦大学高分子科学系聚合物分子工程国家重点实验室上海 200433
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2021.21156
  CLC：
- Published：20 January 2022，
  
  Published Online：26 August 2021，
  
  Received：20 May 2021，
  
  Accepted：06 June 2021
- 稿件说明：
移动端阅览
史柏扬,王国伟.聚合诱导自组装(PISA)技术的应用研究进展[J].高分子学报,2022,53(01):15-29.

Shi Bo-yang,Wang Guo-wei.Application of Polymerization-induced Self-assembly (PISA) Technology[J].ACTA POLYMERICA SINICA,2022,53(01):15-29.
史柏扬,王国伟.聚合诱导自组装(PISA)技术的应用研究进展[J].高分子学报,2022,53(01):15-29. DOI： 10.11777/j.issn1000-3304.2021.21156.

Shi Bo-yang,Wang Guo-wei.Application of Polymerization-induced Self-assembly (PISA) Technology[J].ACTA POLYMERICA SINICA,2022,53(01):15-29. DOI： 10.11777/j.issn1000-3304.2021.21156.

摘要

聚合诱导自组装(PISA)技术是制备嵌段共聚物纳米自组装体的一种新技术. 相较于传统的嵌段共聚物自组装技术，该技术具有边聚合、边组装的操作简便性特点，同时还具有纳米自组装体形态可控、固含量高(高达50%)等优点，使得聚合物纳米自组装体的规模化生产和应用成为可能. 经过十多年的发展，基于各种“活性”/可控聚合机理和各种配方组合的PISA体系已经被成功实现，PISA技术在各个领域的应用研究也得到了全面的推进. 目前关于PISA中的组装体形态研究已经有不少综述，而针对PISA技术应用方面的综述却鲜有报道. 因此，本文在简要介绍PISA技术的基本原理和发展现状的基础上，重点总结了PISA技术在纳米复合材料、生物医用材料、电池、功能涂料、Pickering乳化剂、纳米结构膜、水凝胶、发光材料等相关领域的研究动态和应用进展. 希望本综述能为PISA领域的研究者提供借鉴，并进一步促进聚合物自组装相关领域的研究进展.

Abstract

The polymerization-induced self-assembly (PISA) has been developed as a versatile technique to prepare the block copolymer-based nano-objects. Compared with the traditional block copolymer-based self-assembly technology

the PISA technology is featured with a polymerization process and a simultaneous self-assembly process

as well as with well-controlled morphologies and high solid content (up to 50 wt%). These advantages have facilitated the large-scale production and application of the nano-objects. Based on the modification of various "living"/controlled polymerization mechanisms and the optimization of various formulations

the PISA technology has been well developed over the past decade. Correspondingly

the application of the PISA technology is also widely used. Up to now

several reviews on the morphology evolution of PISA technology have been presented. However

a comprehensive summary on the application of PISA technique is still needed. In this review

following with a brief introduction on the fundamental principle and the status of PISA technology

the application of PISA in nanocomposite materials

biomedical materials

batteries

functional coatings

Pickering emulsifiers

nanostructured membranes

hydrogels

luminescent materials

and other fields will be focused and summarized. This summary is hoped to depict a comprehensive outline of PISA technology in recent years and to prompt the development of the self-assembly technology in interdisciplinary field.

关键词

聚合诱导自组装(PISA)嵌段共聚物纳米自组装体

Keywords

Polymerization-induced self-assembly (PISA)Block copolymerNano-objects

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