Structured Liquids: Design, Construction and Applications

Wei-xiao Feng; Thomas P. Russell; Shao-wei Shi

doi:10.11777/j.issn1000-3304.2023.23300

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Structured Liquids: Design, Construction and Applications

Feature Article | 更新时间：2024-09-20

- Structured Liquids: Design, Construction and Applications
- Acta Polymerica Sinica Vol. 55, Issue 5, Pages: 485-508(2024)
- 作者机构：
  
  1.北京化工大学化工资源有效利用国家重点实验室北京软物质科学与工程高精尖创新中心北京 100029
  2.Department of Polymer Science and Engineering， University of Massachusetts， Amherst， Massachusetts 01003
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2023.23300
  CLC：
- Published：20 May 2024，
  
  Published Online：25 March 2024，
  
  Received：29 December 2023，
  
  Accepted：17 February 2024
- 稿件说明：
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封维潇, Thomas P. Russell, 史少伟. 结构化液体的设计、构筑与应用. 高分子学报, 2024, 55(5), 485-508

Feng, W. X.; Russell, T. P. ; Shi, S. W. Structured liquids: design, construction and applications. Acta Polymerica Sinica, 2024, 55(5), 485-508
封维潇, Thomas P. Russell, 史少伟. 结构化液体的设计、构筑与应用. 高分子学报, 2024, 55(5), 485-508 DOI： 10.11777/j.issn1000-3304.2023.23300.

Feng, W. X.; Russell, T. P. ; Shi, S. W. Structured liquids: design, construction and applications. Acta Polymerica Sinica, 2024, 55(5), 485-508 DOI： 10.11777/j.issn1000-3304.2023.23300.

摘要

结构化液体是近年来基于二元流体体系，利用固体粒子液/液界面自组装和堵塞相变构筑的一类非平衡态软物质材料，兼具固体的结构稳定性和液体的流动性. 然而，受限于组装基元和成型方法，制备具有精准结构的智能结构化液体及衍生功能材料仍面临挑战. 我们课题组在该领域开展了大量研究工作，在发展界面调控新机制，制备液体/固体新材料，以及实现材料器件新突破等方面取得了系列创新成果. 本专论从固体粒子界面自组装机制出发，重点阐述了一种利用纳米粒子和聚合物液/液界面共组装制备纳米粒子表面活性剂，进而构筑结构化液体的普适策略; 总结归纳了结构化液体在响应性调控、高效精准构筑以及功能材料制备等方面的研究进展; 并对该领域面临的机遇和挑战做出展望.

Abstract

Structured liquids are a new type of non-equilibrium soft materials constructed by the assembly and jamming of solid particles at the liquid/liquid interface

combining the structural stability of solids with the fluidity of liquids. However

the preparation of smart structured liquids and derived functional materials with precise structures is still challenging

due to the lacking of suitable building blocks and manufacturing methods. Our group has carried out a great deal of research work in this field

and has achieved a series of significant results in the development of new self-assembly mechanism at the interface

the preparation of new liquid/solid materials

and the construction of novel devices with advanced functions. In this review

we highlight a generalized strategy for the preparation of structured liquids by using the formation

assembly and jamming of nanoparticle surfactants

in which nanoparticle surfactants are generated by the co-assembly between nanoparticles and polymeric ligands at the liquid/liquid interface. We first introduce the self-assembly mechanism of solid particles at the liquid/liquid interface. Then we summarize the progress in the construction of structured liquids and derived materials. Finally

we provide an outlook of the opportunities and challenges in this field.

关键词

结构化液体纳米粒子表面活性剂液/液界面自组装

Keywords

Structured liquidsNanoparticle surfactantsLiquid/liquid interfaceSelf-assembly

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