Component Optical Regulation for High-efficiency and Stable Monolithic All-inorganic Perovskite/Organic Tandem Solar Cells

Ji-xiang Yuan; Hai-di Yang; Ruo-peng Zhang; Peng-peng Dong; Wei-jie Chen; Yao-wen Li

doi:10.11777/j.issn1000-3304.2025.25305

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Component Optical Regulation for High-efficiency and Stable Monolithic All-inorganic Perovskite/Organic Tandem Solar Cells

Research Article | 更新时间：2026-05-08

- Component Optical Regulation for High-efficiency and Stable Monolithic All-inorganic Perovskite/Organic Tandem Solar Cells
  增强出版
- Acta Polymerica Sinica Vol. 57, Issue 5, Pages: 1023-1033(2026)
- 作者机构：
  
  1.苏州大学材料与化学化工学部仿生材料与界面科学中心苏州市新型半导体光电材料与器件重点实验室苏州大学先进光电材料重点实验室苏州 215123
  2.苏州大学江苏省先进负碳技术重点实验室苏州 215123
- 作者简介：
  
  Ruo-peng Zhang, E-mail: zhangruopeng@suda.edu.cn
  Wei-jie Chen, E-mail: wjchen@suda.edu.cn
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2025.25305
  CLC：
- CSTR：32057.14.GFZXB.2025.7538
- Received：19 November 2025，
  
  Accepted：12 December 2025，
  
  Online First：27 January 2026，
  
  Published：20 May 2026
- 稿件说明：
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袁吉祥, 杨海迪, 张若鹏, 董鹏鹏, 陈炜杰, 李耀文. 组分光学调控实现高效稳定全无机钙钛矿/有机叠层太阳能电池. 高分子学报, 2026, 57(5), 1023-1033.

Yuan, J. X.; Yang, H. D.; Zhang, R. P.; Dong, P. P.; Chen, W. J.; Li, Y. W. Component optical regulation for high-efficiency and stable monolithic all-inorganic perovskite/organic tandem solar cells. Acta Polymerica Sinica (in Chinese), 2026, 57(5), 1023-1033.
袁吉祥, 杨海迪, 张若鹏, 董鹏鹏, 陈炜杰, 李耀文. 组分光学调控实现高效稳定全无机钙钛矿/有机叠层太阳能电池. 高分子学报, 2026, 57(5), 1023-1033. DOI： 10.11777/j.issn1000-3304.2025.25305. CSTR： 32057.14.GFZXB.2025.7538.

Yuan, J. X.; Yang, H. D.; Zhang, R. P.; Dong, P. P.; Chen, W. J.; Li, Y. W. Component optical regulation for high-efficiency and stable monolithic all-inorganic perovskite/organic tandem solar cells. Acta Polymerica Sinica (in Chinese), 2026, 57(5), 1023-1033. DOI： 10.11777/j.issn1000-3304.2025.25305. CSTR： 32057.14.GFZXB.2025.7538.

摘要

全无机钙钛矿/有机叠层太阳能电池(TSCs)有望突破单结Shockley-Queisser极限. 然而，宽带隙钙钛矿前电池的滤光效应会引起光生电流失配及有机后电池载流子动力学改变，造成严重的能量损失，限制了叠层器件性能的提升. 本研究提出一种组分光学调控策略：通过提高有机体异质结(BHJ)中的受体组分含量，增强了薄膜在滤光条件下的近红外光子捕获能力，使前后电池光电流更加平衡，有效地降低了TSCs的光学损失. 此外，该策略还可提供额外的电子传输路径，平衡了空穴与电子迁移率，进而抑制双分子复合、促进激子解离. 最终实现叠层太阳能电池23.65%的光电转化效率、2.17 V的开路电压和79.58%的填充因子. 此外，该器件展现出良好的工作稳定性，在1000 h持续运行后仍保持初始效率的88%，并且紫外光稳定性良好.

Abstract

Monolithic all-inorganic perovskite/organic tandem solar cells (TSCs) are highly promising for surpassing the single-junction Shockley-Queisser limit. However

the practical performance of such TSCs is often constrained by significant energy losses

primarily stemming from imbalanced photocurrent generation and altered charge carrier dynamics in the organic rear subcell under the optical filtering effect of the wide-bandgap perovskite front cell. Herein

we proposed a component optical regulation strategy to tackle this challenge. By strategically increasing the acceptor content in the organic bulk-heterojunction (BHJ)

we concurrently enhanced the near-infrared photon capture and optimize the charge carrier dynamics under filtered illumination. This approach provided additional electron transport pathways

effectively balancing the hole and electron mobility

which in turn suppressed bimolecular recombination and promoted exciton dissociation

as verified by transient absorption spectroscopy. Consequently

the optimized TSC achieved a champion power conversion efficiency of 23.65% with an ultrahigh open-circuit voltage of 2.17 V and an impressive fill factor of 79.58%. Moreover

the device exhibited remarkable operational stability

retaining 88% of its initial efficiency after 1000 h

and superior UV resilience.

关键词

Keywords

references

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