生物基可聚合单体及其聚合物制备与性能研究进展

陈沁; 杜杰毫; 谢海波; 赵宗保; 郑强

doi:10.11777/j.issn1000-3304.2016.16154

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生物基可聚合单体及其聚合物制备与性能研究进展

综述 | 更新时间：2021-03-19

- 生物基可聚合单体及其聚合物制备与性能研究进展
- Studies on Preparation and Properties of Bio-based Polymeric Monomers and Their Bio-based Polymers
- 高分子学报 2016年第10期页码：1330-1358
- 作者机构：
  
  1.贵州大学材料与冶金学院高分子材料与工程系贵阳 550025
  2.中国科学院大连化学物理研究所大连 116023
- 作者简介：
  
  谢海波,E-mail:hbxie@dicp.ac.cn Hai-bo Xie,E-mail:hbxie@dicp.ac.cn
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2016.16154
  中图分类号：
- 纸质出版日期：2016-10，
  
  收稿日期：2016-5-11，
  
  修回日期：2016-6-20，
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陈沁, 杜杰毫, 谢海波, 赵宗保, 郑强. 生物基可聚合单体及其聚合物制备与性能研究进展[J]. 高分子学报, 2016,(10):1330-1358.

Chen Qin, Du Jie-hao, Xie Hai-bo, Zhao Zong-bao, Zheng Qiang. Studies on Preparation and Properties of Bio-based Polymeric Monomers and Their Bio-based Polymers[J]. Acta Polymerica Sinica, 2016,(10):1330-1358.
陈沁, 杜杰毫, 谢海波, 赵宗保, 郑强. 生物基可聚合单体及其聚合物制备与性能研究进展[J]. 高分子学报, 2016,(10):1330-1358. DOI： 10.11777/j.issn1000-3304.2016.16154.

Chen Qin, Du Jie-hao, Xie Hai-bo, Zhao Zong-bao, Zheng Qiang. Studies on Preparation and Properties of Bio-based Polymeric Monomers and Their Bio-based Polymers[J]. Acta Polymerica Sinica, 2016,(10):1330-1358. DOI： 10.11777/j.issn1000-3304.2016.16154.

摘要

对化石资源的过渡开采导致了严重的能源危机及环境问题，发展生物基聚合物代替石油基聚合物是缓解当前危机的有效途径之一.本文总结了国内外研究人员在生物基聚合物研究领域的最新进展，重点介绍了生物基脂肪族单体、芳香族单体的制备，包括生物基羧酸单体、生物基二醇单体、生物基烃类单体、呋喃基单体、香草醛单体，比较了不同制备方法的选择性及产率；采用传统及新型的聚合方法，如熔融缩聚、自由基聚合、酶催化聚合等，可以将生物基单体转化为各种生物基聚合，包括聚酯、聚酰胺、聚碳酸酯等，并比较了聚合条件对生物基聚合物制备的影响.生物基聚合物具有优良的机械性能及热性能，并展现出各种优异特性，如形状记忆、自修复功能等，有望代替传统的石油基聚合物.最后，对国内外生物基质聚合物的前景做了展望.

Abstract

The search for sustainable resource for polymers production have been obtained much attentions due to the over exploration of fossil resources and environment problems arisen from the use of petroleum based polymeric materials.The modern biorefinery produced a spectrum of biobased chemicals

which can be further upgraded into polymeric monomers for polymer synthesis.This review summarized the latest progress in the synthesis of biobased polymeric monomers from renewable resources such as carbohydrates

lignocellulose and plan oils.According to their structure

those biobased polymeric monomers can be categorised into aliphatic monomers and aromatic monomers including acids

diols

furyl and vanillic monomers.Various strategies

such as catalytic process and fementaion process

were compared in terms of selectivity

yield and feasibility of target biobased monomers.Those biobased monomers can be directly employed as feedstock to prepare biobased polymers

such as polyesters

polyamides

polycarbonates

polyurethanes and polyethers.Besides

both the traditional and novel polymerization processes can be adopted to prepare biobased polymers

such as catalyst free melt condensation

radical polymerization

photocuring process

proton transfer polymerization and enzymatic polycondensations.The influence of various heating methods

catalyst loading

mole ratio

reaction time and temperature to prepare biobased polymers were compared.Those biobased polymers exhibit excellent mechanical and thermal properties and promising properties such as shape memory effect

self-healing properties and bacteria clearing effect

which revealed great potential to replace the petroleum based polymers.Finally

the future development of bio-based polymers has also discussed.

关键词

催化生物炼制生物基单体生物基聚合物热性能机械性能

Keywords

Catalytic biorefineryBio-based monomersBio-based polymersThermal propertiesMechanical properties

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