两性离子水凝胶的研究进展

李平; 曾良鹏; 郭宏磊; 郭辉; 李伟华

doi:10.11777/j.issn1000-3304.2020.20124

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两性离子水凝胶的研究进展

综述 | 更新时间：2021-01-26

- 两性离子水凝胶的研究进展
- Research Progress in Zwitterionic Hydrogels
- 高分子学报 2020年51卷第12期页码：1307-1320
- 作者机构：
  
  中山大学化学工程与技术学院　珠海 519082
- 作者简介：
  
  [ "郭宏磊，男，1986年生. 中山大学化学工程与技术学院副教授，硕士生导师，2016年于日本北海道大学获生命科学博士学位. 2019年3月受聘中山大学“百人计划”副教授. 主要从事软物质材料、功能高分子材料和金属腐蚀防护涂层等方向的研究" ]
  [ "郭辉，男，1987年生，现任中山大学化学工程与技术学院副教授. 2009年和2012年于上海交通大学获分别学士和硕士学位；2015年于法国巴黎第六大学获材料物理与化学方向博士学位，2019年2月受聘中山大学“百人计划”副教授. 获国家自然科学基金委青年科学基金、广东省自然科学基金等项目，主要研究方向为高分子凝胶、智能软物质材料等" ]
- 基金信息：
  
  国家自然科学基金 (基金号 51903253)和广东省自然科学基金(基金号 2019A1515011150)资助项目
- DOI：10.11777/j.issn1000-3304.2020.20124
  中图分类号：
- 纸质出版日期：2020-10-21，
  
  网络出版日期：2020-8-18，
  
  收稿日期：2020-5-15，
  
  修回日期：2020-6-8，
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李平, 曾良鹏, 郭宏磊, 郭辉, 李伟华. 两性离子水凝胶的研究进展[J]. 高分子学报, 2020,51(12):1307-1320.

Ping Li, Liang-peng Zeng, Hong-lei Guo, Hui Guo, Wei-hua Li. Research Progress in Zwitterionic Hydrogels[J]. Acta Polymerica Sinica, 2020,51(12):1307-1320.
李平, 曾良鹏, 郭宏磊, 郭辉, 李伟华. 两性离子水凝胶的研究进展[J]. 高分子学报, 2020,51(12):1307-1320. DOI： 10.11777/j.issn1000-3304.2020.20124.

Ping Li, Liang-peng Zeng, Hong-lei Guo, Hui Guo, Wei-hua Li. Research Progress in Zwitterionic Hydrogels[J]. Acta Polymerica Sinica, 2020,51(12):1307-1320. DOI： 10.11777/j.issn1000-3304.2020.20124.

摘要

两性离子水凝胶是一类具有独特结构特点的软物质材料，其三维高分子网络中富含阴阳离子基团，同时在宏观上表现出电中性. 基于其结构的特殊性，两性离子水凝胶在近十余年来得到了广泛关注和深入研究. 本综述系统介绍了两性离子水凝胶的功能特点，详细总结了两性离子水凝胶在生物医学、凝胶电解液、传感器和驱动器等领域的应用，深入解析了制约两性离子水凝胶应用的主要因素并总结展望了两性离子水凝胶在未来发展中面临的挑战与机遇.

Abstract

Zwitterionic hydrogels have received considerable attention owing to their characteristic structures and properties. Bearing high density of oppositely charged groups within polymer networks at the micro-scale

the zwitterionic hydrogels exhibit a macroscopic electro-neutrality. As a result

the soft matter exhibits various specific features

such as high hydrophilicity owing to their dense charged groups

“anti-polyelectrolyte behavior” due to salt clearable associations between oppositely charged groups

and UCST-type thermo-responsiveness as a result of temperature-sensitive polymer inner and inter-chain associations. In this review

the unique properties of the materials are described at first

and their potential applications including biomedicine

gel polymer electrolyte

sensor

and actuator are subsequently illustrated in detail. Thereafter

the possible constraints that hinder their current practical application are well discussed. The difficulty in monomer synthesis

the relatively poor chemical stability against long term hydrolysis and oxidization in aqueous media

and unsatisfactory mechanical performance are three main plausible reasons. Developing zwitterionic hydrogels with ameliorated chemical structures effectively enhances their chemical stability

while the exploration of polyzwitterionic composite hydrogels with nanoparticles is a possible way to figure out the existing drawback of poor mechanical performance. In the end

current status as well as future prospect of the zwitterionic hydrogels are finely presented.

关键词

两性离子水凝胶生物医学凝胶电解液传感器驱动器

Keywords

ZwitterionicHydrogelBiomedicineGel polymer electrolyteSensorActuator

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