聚合物限域和预有序熔体的结晶行为及结构调控

初笑; 闫寿科; 孙晓丽

doi:10.11777/j.issn1000-3304.2021.21036

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聚合物限域和预有序熔体的结晶行为及结构调控

专论 | 更新时间：2021-11-03

- 聚合物限域和预有序熔体的结晶行为及结构调控
- Crystallization Mechanism and Structure Control of Polymers in Confined Space and from Pre-ordered Melt
- 高分子学报 2021年52卷第6期页码：634-645
- 作者机构：
  
  1.北京化工大学材料科学与工程学院化工资源有效利用国家重点实验室　北京 100029
  2.青岛科技大学橡塑材料与工程教育部重点实验室　青岛 266042
- 作者简介：
  
  [ "孙晓丽，女，1982年生. 北京化工大学材料科学与工程学院教授，2003~2009年在中国科学院化学研究所获得博士学位；2006~2008年在马普高分子研究所博士联合培养；2009~2011年在日本关西学院大学从事博士后研究. 2012~2017年任北京化工大学副教授；2018年至今任北京化工大学教授. 曾获“北京化工大学青年百人计划”和“国家基金委优秀青年科学基金”资助. 主要研究方向为聚合物的结晶机制、结构调控及性能研究" ]
- 基金信息：
  
  国家自然科学基金(基金号 22022501)资助项目
- DOI：10.11777/j.issn1000-3304.2021.21036
  中图分类号：
- 纸质出版日期：2021-6-3，
  
  网络出版日期：2021-5-6，
  
  收稿日期：2021-2-1，
  
  修回日期：2021-3-4，
扫描看全文
初笑, 闫寿科, 孙晓丽. 聚合物限域和预有序熔体的结晶行为及结构调控[J]. 高分子学报, 2021,52(6):634-645.

Xiao Chu, Shou-ke Yan, Xiao-li Sun. Crystallization Mechanism and Structure Control of Polymers in Confined Space and from Pre-ordered Melt[J]. Acta Polymerica Sinica, 2021,52(6):634-645.
初笑, 闫寿科, 孙晓丽. 聚合物限域和预有序熔体的结晶行为及结构调控[J]. 高分子学报, 2021,52(6):634-645. DOI： 10.11777/j.issn1000-3304.2021.21036.

Xiao Chu, Shou-ke Yan, Xiao-li Sun. Crystallization Mechanism and Structure Control of Polymers in Confined Space and from Pre-ordered Melt[J]. Acta Polymerica Sinica, 2021,52(6):634-645. DOI： 10.11777/j.issn1000-3304.2021.21036.

摘要

高分子物理领域的挑战性难题之一是调控高分子的结晶行为. 高分子结构具有多尺度的特点，且易受到各种本征因素以及加工过程中引入的外场与受限作用的影响. 高分子的结晶过程复杂多变，为避免最终产品性能的良莠不齐，促进高分子材料的实际生产和应用，需要建立高分子结构与性能的直接关系并实现对高分子结晶结构的精细化调控. 本文以几种典型高分子为例，重点阐述了我们课题组在有关薄膜和纳米孔道构筑的限域空间与分子链预有序熔体对高分子结晶行为的影响、相关结晶结构调控机制以及结构-性能关系等方面的研究工作，阐明了聚合物多层次结构调控领域存在的科学问题，并展望了其未来发展方向.

Abstract

Polymer crystallization still remains one of the most important and challenging issues of polymer physics. As crystallization process of polymers is complex and variable under different conditions

it is necessary to establish the direct structure-property relationship of polymers and realize the purposeful crystalline structure regulation of polymers. Herein

taking several typical polymers as examples

we summarize the research progresses on the crystallization behavior and the multiscale structure control of semi-crystalline polymers. Based on the research work of our group

the emphasis of this feature article is especially focused on the crystallization and structure regulation of polymers in confined spaces

e.g.

in ultrathin film and nanoporous channels

and from preordered melts. The crystallization mechanism is discussed. In addition

challenging and scientific problems existing in the field of polymer crystallization and multiscale structure regulation

which may guide the future development direction of this field

have been described.

关键词

聚合物结晶多层次结构调控受限作用熔体预有序

Keywords

Polymer crystallizationMultiscale structure regulationConfinement effectPre-ordered melting molecular chains

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