倍增型有机光电探测器的研究进展

王健; 赵子进; 杨凯旋; 陈亮; 刘明; 张福俊

doi:10.11777/j.issn1000-3304.2021.21328

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倍增型有机光电探测器的研究进展

综述 | 更新时间：2024-10-08

- 倍增型有机光电探测器的研究进展
- A Critical Review on Photomultiplication Type Organic Photodetectors
- 高分子学报 2022年53卷第4期页码：331-353
- 作者机构：
  
  1.泰山学院物理与电子工程学院泰安 271000
  2.北京交通大学光信息与发光技术教育部重点实验室北京 100044
- 作者简介：
  
  [ "王健，男，1986年生. 2016年毕业于北京交通大学，获工学博士学位，导师张福俊教授. 2016年入职泰山学院，次年破格晋升教授. 2017、2020年先后获得国家自然科学基金青年项目、面上项目立项资助，近4年以第一或通讯作者在《Advanced Functional Materials》《Sustainable Energy and Fuels》《Journal of Materials Chemistry C》《ACS Applied Materials & Interfaces》等期刊发表论文20余篇. 现主要从事三元有机光伏器件的工作机制及性能改善、倍增型有机光电探测器性能改善与成像应用的研究." ]
  [ "张福俊，男，1975年生. 2007年毕业于北京交通大学，获博士学位. 2007年入职北京交通大学，目前教授三级岗、博士生导师. 一项成果入选2017年中国光学十大进展，主持完成的倍增型有机光电探测器的研究成果荣获北京市科学技术三等奖. 在影响因子15以上的期刊上发表论文近30篇，连续3年入选英国皇家化学学会高被引中国作者，入选全球顶尖前10万科学家名单. 主要从事三元有机光伏材料与器件物理、倍增型有机光电探测器的工作." ]
- 基金信息：
  
  国家自然科学基金(基金号 ┣61975006);62075155┫;山东省自然科学基金(基金号 ZR2021MF077)
- DOI：10.11777/j.issn1000-3304.2021.21328
  中图分类号：
- 纸质出版日期：2022-04-20，
  
  网络出版日期：2022-01-26，
  
  收稿日期：2021-10-30，
  
  录用日期：2021-12-09
- 稿件说明：
移动端阅览
王健,赵子进,杨凯旋等.倍增型有机光电探测器的研究进展[J].高分子学报,2022,53(04):331-353.

Wang Jian,Zhao Zi-jin,Yang Kai-xuan,et al.A Critical Review on Photomultiplication Type Organic Photodetectors[J].ACTA POLYMERICA SINICA,2022,53(04):331-353.
王健,赵子进,杨凯旋等.倍增型有机光电探测器的研究进展[J].高分子学报,2022,53(04):331-353. DOI： 10.11777/j.issn1000-3304.2021.21328.

Wang Jian,Zhao Zi-jin,Yang Kai-xuan,et al.A Critical Review on Photomultiplication Type Organic Photodetectors[J].ACTA POLYMERICA SINICA,2022,53(04):331-353. DOI： 10.11777/j.issn1000-3304.2021.21328.

摘要

介绍了倍增型有机光电探测器的发展、工作机理、性能调控及相关的应用探索. 2015年张福俊课题组以单载流子传输通道的给受体混合(质量比约为100:1)薄膜为有源层，率先报道了界面附近受陷电子诱导空穴隧穿注入的倍增型有机光电探测器，并抑制了器件的暗电流密度. 通过优化有源层厚度调控了界面附近受陷电荷的体分布，制备出超窄响应的倍增型有机光电探测器，并提出载流子注入窄化的新概念. 利用三元策略及双层策略，制备出了宽响应倍增型有机光电探测器. 利用光子俘获层调控器件的响应范围，以及利用倍增层获得了较大的外量子效率，将二极管型与倍增型器件的优势集中在一个器件中. 引入光学调控层或将宽带隙材料引入有源层中，调控界面附近受陷电子分布，优化了器件的光谱形状，进而制备出响应光谱宽且平的倍增型有机光电探测器. 将制备的倍增型有机光电探测器应用到心率监测、单像素成像及光开关等领域，取得较好的应用成果.

Abstract

This review systematically summarizes the development

working mechanism

performance optimization and relevant application exploration of photomultiplication type organic photodetectors (PM-OPDs). In 2015

Prof. Fujun Zhang's group firstly reported PM-OPDs on the basis of active layers with single carrier transport channels. Electron traps are formed with acceptor surrounded by donor in active layers with the weight ratio of donor to acceptor as about 100:1. The working mechanism of PM-OPDs is attributed to hole tunneling injection assisted by interfacial trapped electron. Dark current density of PM-OPDs can be well suppressed due to the single carrier transport in active layers with rather less acceptor. New concept of "charge injection narrowing" was firstly proposed to prepare ultra-narrowband PM-OPDs

which is realized by adjusting thickness of active layers to control interfacial trapped electron distribution. Broadband PM-OPDs can be obtained

via

ternary strategy or double-layer scheme. Double-layer scheme consists of one absorption layer and one PM layer

which are individually employed to tune spectral response range of PM-OPDs and achieve external quantum efficiency greater than 100%. The advantages of photodiode type photodetectors and PM-OPDs can be integrated into one device by employing double-layer scheme. PM-OPDs with broad and flat spectral response can be achieved

via

optimizing interfacial trapped electron distribution

which can be regulated by inserting optical field adjusting layer or incorporating wide bandgap semiconductor materials into active layers. The PM-OPDs have been successfully applied in many fields

such as heart rate monitoring

single pixel imaging and optical switch. The successful practical applications indicate good development prospect of PM-OPDs.

关键词

倍增型有机光电探测器隧穿注入外量子效率响应范围

Keywords

Photomultiplication type organic photodetectorsTunnelling injectionExternal quantum efficiencySpectral range

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