氢键交联超分子聚合物材料：从结构性能到功能应用

王振宇; 牛文文; 张卓强; 刘小孔

doi:10.11777/j.issn1000-3304.2023.23064

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氢键交联超分子聚合物材料：从结构性能到功能应用

专论 | 更新时间：2023-08-21

- 氢键交联超分子聚合物材料：从结构性能到功能应用
- Hydrogen-bonded Supramolecular Polymeric Materials: From Structure and Performance to Functionality and Application
- 高分子学报 2023年54卷第9期页码：1272-1289
- 作者机构：
  
  超分子结构与材料国家重点实验室吉林大学化学学院长春 130012
- 作者简介：
  
  [ "刘小孔，男，1985年生. 现任吉林大学化学学院/超分子结构与材料国家重点实验室教授、博士生导师；分别于2005和2010年在吉林大学化学学院获得学士和博士学位，师从孙俊奇教授；在攻读博士学位期间和博士毕业后，分别在德国马普胶体与界面研究所、澳大利亚南澳大学、加拿大阿尔伯塔大学从事研究工作；2017年入选国家高层次青年人才计划并受聘吉林大学教授，主要研究方向包括超分子聚合物材料、柔性电子材料与器件、自清洁涂层涂料等." ]
- 基金信息：
  
  国家自然科学基金(基金号 22275069)
- DOI：10.11777/j.issn1000-3304.2023.23064
  中图分类号：
- 纸质出版日期：2023-09-20，
  
  网络出版日期：2023-06-04，
  
  收稿日期：2023-03-19，
  
  录用日期：2023-04-18
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王振宇,牛文文,张卓强等.氢键交联超分子聚合物材料：从结构性能到功能应用[J].高分子学报,2023,54(09):1272-1289.

Wang Zhen-yu,Niu Wen-wen,Zhang Zhuo-qiang,et al.Hydrogen-bonded Supramolecular Polymeric Materials: From Structure and Performance to Functionality and Application[J].ACTA POLYMERICA SINICA,2023,54(09):1272-1289.
王振宇,牛文文,张卓强等.氢键交联超分子聚合物材料：从结构性能到功能应用[J].高分子学报,2023,54(09):1272-1289. DOI： 10.11777/j.issn1000-3304.2023.23064.

Wang Zhen-yu,Niu Wen-wen,Zhang Zhuo-qiang,et al.Hydrogen-bonded Supramolecular Polymeric Materials: From Structure and Performance to Functionality and Application[J].ACTA POLYMERICA SINICA,2023,54(09):1272-1289. DOI： 10.11777/j.issn1000-3304.2023.23064.

摘要

高分子材料的大量消耗与持续积累已经在全球范围内造成了严重的环境污染与资源浪费. 发展可修复、可循环、可降解和可回收的新一代高分子材料是解决上述挑战的根本途径. 基于动态可逆的非共价键将聚合物链段进行交联可以有效地构建这些材料. 本专论系统总结了我们课题组在氢键交联超分子聚合物材料方面的系列研究进展. 基于多重氢键的协同性与动态性、氢键与动态共价键的协同，以及材料微相结构的调控，发展了系列兼具高强度与高韧性的超分子聚合物材料，实现了材料的修复、循环、降解与回收；不仅突破了非共价交联高分子材料力学性能弱的瓶颈，而且化解了高分子材料强度与韧性的矛盾. 相关研究为发展传统高分子材料的可持续替代品提供了新的思路. 同时，发展了系列基于氢键交联的功能超分子聚合物材料，展示了其在柔性电子、固态锂电池及水下黏合剂等方面的应用.

Abstract

The huge consumption of polymeric materials in the world has led to a dramatic increase in plastic waste

which has caused pervasive environmental pollution and severe waste of material resources. Crosslinking the polymer segments by noncovalent bonds is an effective method for developing healable

degradable

and recyclable polymeric materials

which could be a fundamental solution to the global plastic waste crisis. However

the noncovalently crosslinked polymeric materials usually exhibit low mechanical robustness

hindering their practical applications. In this feature article

we summarized the recent research progress of our group on hydrogen-bonded supramolecular polymeric materials with high mechanical robustness and various functionalities. Based on the synergistic effect of high-density hydrogen bonds

the cooperation of hydrogen bonds and dynamic covalent bonds

and the regulation of the microstructures of the polymeric materials

we have developed a series of healable

degradable

and recyclable supramolecular polymer materials that simultaneously possess high strength and high toughness. Our results not only break the bottleneck of poor mechanical properties of noncovalently crosslinked polymeric materials

but also reconcile the mutual exclusiveness between the strength and toughness of polymer materials. These studies provide new ideas for the development of the high-performance sustainable alternatives to traditional polymer materials. Moreover

we have developed a series of hydrogen-bonded functional supramolecular polymeric materials

and their applications in flexible electronic devices

solid-state lithium batteries

and underwater adhesives are also introduced in this feature article.

关键词

超分子高分子材料氢键力学性能可持续发展

Keywords

Supramolecular materialsPolymeric materialsHydrogen bondsMechanical propertiesSustainability

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