Recent Advances in Second Order Nonlinear Optical Polymers with Dendritic Structure

Li Zhong-an; Li Zhen

doi:10.11777/j.issn1000-3304.2017.16274

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Recent Advances in Second Order Nonlinear Optical Polymers with Dendritic Structure

Feature Articles | 更新时间：2021-05-18

- Recent Advances in Second Order Nonlinear Optical Polymers with Dendritic Structure
- Acta Polymerica Sinica Issue 2, Pages: 155-177(2017)
- 作者机构：
  
  武汉大学化学与分子科学学院武汉 430072
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2017.16274
  CLC：
- Published：20 February 2017，
  
  Received：6 September 2016，
  
  Revised：13 November 2016，
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Li Zhong-an, Li Zhen. Recent Advances in Second Order Nonlinear Optical Polymers with Dendritic Structure. [J]. Acta Polymerica Sinica (2):155-177(2017)
DOI：

Li Zhong-an, Li Zhen. Recent Advances in Second Order Nonlinear Optical Polymers with Dendritic Structure. [J]. Acta Polymerica Sinica (2):155-177(2017) DOI： 10.11777/j.issn1000-3304.2017.16274.

摘要

树状分子是指一类结构高度支化的大分子或高分子化合物，其独特的三维纳米球形结构、分子内空腔以及大量富集的表面基团，可产生诸多特殊且有趣的功能及光物理性质，在化学、生物和材料等领域获得了广泛的关注和研究.本文主要综述了我们课题组在具有枝状结构二阶非线性光学高分子方面的研究进展，重点介绍了如何通过合理分子设计，发展不同类型枝状拓扑结构以有效提高材料的综合性能，并展望了该领域的今后发展趋势.

Abstract

Dendritic molecules are a class of highly branched macromolecules and/or polymers having a three-dimensional

nanosized globular architecture with intramolecular cavity and numerous surface functional groups. These unique structural features can endow dendritic molecules with a lot of particular and interesting functionalities and photophysical properties

making them very attractive in many areas including chemistry

biology

materials

and so on. In the past 30 years

organic/polymeric second-order nonlinear optical (NLO) materials have been widely investigated due to their great potential in telecommunications

computing

terahertz generation

detection

and many other photonic applications. So far

one of the major challenges encountered in this field is how to translate high molecular nonlinearities (μ

) of chromophores into large macroscopic material nonlinearities (i.e. second harmonic generation coefficient

d33) efficiently

due to the strong intermolecular dipole-dipole interactions between chromophore moieties

which can make their poling induced noncentrosymmetric alignment a daunting task. According to the site-isolation principle

the dendritic structure has been well-recognized as the next generation molecular topology to modify chromophores into the ideal spherical shape that can minimize the dipole-dipole interactions significantly to improve the poling efficiency. From 2006

our group has done many systematic researches in this field with an attempt to better understand the structure-properties relationship of NLO polymeric materials. In this review

after a brief introduction of dendritic molecules and second order nonlinear optics

we will summarize our recent research work on second order NLO polymers with dendritic structure

including high generation dendrimers

hyperbranched polymers and dendronized hyperbranched polymers (a new polymer model combining hyperbranched polymer and dendrimer). We mainly focus on the discussion how to rationally design and tailor the topological structures of the dendritic NLO polymers that can significantly enhance their comprehensive material performance through several molecular design strategies such as "suitable isolation group"

"isolation chromophore" and the Ar-ArF self-assembly. Finally

a short outlook for future opportunities in advancing this field is also presented.

关键词

树枝状高分子非线性光学拓扑结构树枝状超支化高分子

Keywords

Dendritic polymersNonlinear opticsTopological structureDendronized hyperbranched polymer

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College of Chemistry, Jilin University

Department of Polymer Science and Engineering, University of Science and Technology of China

The State Key Laboratory of Molecular Engineering of Polymers, Department of Macromolecular Science, Fudan University

School of Polymer Science and Engineering, Qingdao University of Science and Technology

Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University

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