Progress in the Study of Microgel Colloidal Crystals

Guan Ying; Zhang Yong-jun

doi:10.11777/j.issn1000-3304.2017.17169

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Progress in the Study of Microgel Colloidal Crystals

Reviews | 更新时间：2021-01-26

- Progress in the Study of Microgel Colloidal Crystals
- Acta Polymerica Sinica Issue 11, Pages: 1739-1752(2017)
- 作者机构：
  
  南开大学化学学院天津 300071
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2017.17169
  CLC：
- Published：20 November 2017，
  
  Received：29 June 2017，
  
  Revised：6 September 2017，
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Guan Ying, Zhang Yong-jun. Progress in the Study of Microgel Colloidal Crystals. [J]. Acta Polymerica Sinica (11):1739-1752(2017)
DOI：

Guan Ying, Zhang Yong-jun. Progress in the Study of Microgel Colloidal Crystals. [J]. Acta Polymerica Sinica (11):1739-1752(2017) DOI： 10.11777/j.issn1000-3304.2017.17169.

摘要

Poly（

-isopropylacrylamide）（PNIPAM）微凝胶粒子是一种软的胶体粒子.和单分散的SiO

、PS、PMMA等硬的胶体粒子一样，单分散的PNIPAM微凝胶粒子也可以自组装成为高度有序的胶体晶体.微凝胶粒子软物质的特性及其对外部刺激的响应性赋予其不同于硬球的组装行为.微凝胶胶体晶体的高度有序结构及其刺激响应性使其在诸多领域有重要用途.本文分别介绍了三维及二维微凝胶胶体晶体组装的研究进展，并对已开发的基于微凝胶胶体晶体的应用进行了总结.

Abstract

Monodisperse hard colloid particles

such as SiO

PS and PMMA colloids

can self-assemble into highly ordered colloidal crystals

and have important applications in a wide range of fields

including photonic crystals

surface patterning

chemical and biosensing

etc

. Monodisperse PNIPAM microgel

a soft colloid

can also self-assemble into highly ordered colloidal crystals. Monodisperse PNIPAM microgel particles with size varying from tens of nanometers to several microns can be facilely synthesized by free-radical precipitation polymerization. Thanks to its soft nature and ability to respond to external stimuli

PNIPAM microgels exhibit self-assembly behavior different from that of hard colloids. The volume fraction

which is a key parameter for the crystallization of a colloidal dispersion

can be facilely tuned by temperature. In addition

because of the soft nature of the microgel spheres

microgel colloidal crystals are intrinsically defect-tolerant. Therefore large arrays of colloidal crystals with highly ordered structure can be facilely fabricated from these spheres. The highly ordered structure and the unique responsiveness to external stimili also make the microgel colloidal crystals highly promising for applications in various fields. Here we review the progress in the fabrication of both 3D and 2D microgel colloidal crystals. The general features of microgel colloidal crystals

such as crystallization and melting kinetics

and packing structures

were summarized. Emphasis was put on the recent efforts

e.g.

the assembly of binary microgel colloidal crystals

the stabilization of the highly ordered structure of microgel colloidal crystals

the introduction of artificial defects into microgel colloidal crystals

and the assembly of large area

highly ordered 2D microgel colloidal crystals. The applications of microgel colloidal crystals already emerged were also reviewed

including their applications as colloidal atoms to study the process of crystallization and melting of the real crystals

as template to synthesize new materials with ordered structure and microgel clusters with ordered crystalline structure

and optical switcher and sensors.

关键词

微凝胶胶体晶体刺激响应自组装

Keywords

MicrogelsColloidal crystalsStimuli-responsivitySelf-assembly

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State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology

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Shanghai Key Laboratory of Advanced Polymeric Materials, School of Materials Science and Engineering, East China University of Science and Technology

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School of Materials Science and Engineering, East China University of Science and Technology

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