Hydrogen Bonding Interactions Mediated Self-assembly Structures of Multicomponent Block Copolymer Mixtures

Ruey-Chorng Lin; Shiao-Wei Kuo

doi:10.11777/j.issn1000-3304.2018.18020

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Hydrogen Bonding Interactions Mediated Self-assembly Structures of Multicomponent Block Copolymer Mixtures

Reviews | 更新时间：2021-01-26

- Hydrogen Bonding Interactions Mediated Self-assembly Structures of Multicomponent Block Copolymer Mixtures
- Acta Polymerica Sinica Vol. 0, Issue 8, Pages: 1016-1032(2018)
- 作者机构：
  
  台湾中山大学材料与光电科学学系　高雄 80424
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2018.18020
  CLC：
- Published：2018-8，
  
  Received：16 January 2018，
  
  Revised：23 February 2018，
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Ruey-Chorng Lin, Shiao-Wei Kuo. Hydrogen Bonding Interactions Mediated Self-assembly Structures of Multicomponent Block Copolymer Mixtures. [J]. Acta Polymerica Sinica 0(8):1016-1032(2018)
DOI：

Ruey-Chorng Lin, Shiao-Wei Kuo. Hydrogen Bonding Interactions Mediated Self-assembly Structures of Multicomponent Block Copolymer Mixtures. [J]. Acta Polymerica Sinica 0(8):1016-1032(2018) DOI： 10.11777/j.issn1000-3304.2018.18020.

摘要

调控嵌段共聚物共混体系的氢键作用力可应用在光学、电性及生物医用领域，因此吸引了高分子科学家广泛的研究兴趣，它提供了制备新型高分子材料(包含可调性及响应性的功能)的方法. 在此篇综述中，我们整理了各种氢键作用力调控嵌段共聚物共混体系(如嵌段共聚物/低分子量化合物、嵌段共聚物/均聚物及嵌段共聚物/嵌段共聚物混合体系)在固态及液态的自组装行为.

Abstract

Self-assembly from block copolymers is a bottom-up process

a relatively inexpensive and simple approach for the preparation of large-scale nano-patterns. This self-assembly from diblock copolymers is driven by the combination of repulsive and attractive interactions due to the covalent bond linkage. The intrinsic immiscibility or incompatibility among the A or B block segments possesses the repulsive force and then confines into nanoscaled domain through the microphase separation because of the attractive force from the covalent bond linkage of A and B block segments. In general

these diblock copolymers can form different well-defined nanostructures in the bulk state including alternative lamellae

bicontinuous double gyroid

hexagonally packed cylinder

and body-centered cubic (BCC) structures

depending on the relative volume fractions of the block copolymer segments

interaction parameters (

)

and degrees of polymerization (

). However

the preparation of block copolymers with controlled volume fraction would be complicated and time-consuming; thus the diblock copolymers (A-

-B) blending with their homopolymer or low-molecular-weight compound would be an easier method for preparing different self-assembled nanostructures. Therefore

self-assembly nanostructures of block copolymer mixtures through mediated hydrogen bonding interactions have attracted much interest in polymer science because of their potential applications in photonic

electronic and biomedical fields

which could offer the unique possibility to create new functional polymeric materials with tunable and responsive behaviors. In this review article

we describe the self-assembly nanostructure of the block copolymer mixtures including block copolymer/low molecular weight compound

block copolymer/homopolymer

and block copolymer/block copolymer mixtures in bulk and solution states by mediated hydrogen bonding strength. Mediated strength of hydrogen bonding in block copolymer blending with homopolymer or block copolymer could provide order-order phase transition from typical lamellar

double gyroid

cylinder

and BCC spherical structure

even various hierarchical self-assembly structures such as three-phase lamellae

core-shell cylinder

and cylinder in lamellae structures in bulk state. Furthermore

it also possesses the different micellar structures of block copolymer mixtures such as spheres

rods

vesicles

and even large compound micelles in solution state.

关键词

氢键作用力嵌段共聚物共混体系自组装结构

Keywords

Hydrogen bondingBlock copolymerPolymer blendSelf-assembly structures

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College of Chemical Engineering, Fuzhou University

College of Materials Science and Engineering, Nanjing Tech University

State Key Laboratory of Materials-Oriented Chemical Engineering

College of Biotechnology and Pharmaceutical Engineering

Beijing National Laboratory for Molecular Sciences, Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center for Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking University

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