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Further Expansions and Applications of the Principles and Methodology of Non-covalent Connected Micelles
- Acta Polymerica Sinica Vol. 0, Issue 8, Pages: 1048-1065(2018)
- 作者机构：
复旦大学高分子科学系 聚合物分子工程国家重点实验室 上海 200438
- 作者简介：
- 基金信息：
DOI：10.11777/j.issn1000-3304.2018.18064
CLC：Published：2018-8，
Received：14 February 2018，
Revised：10 April 2018，
扫 描 看 全 文
Guo-song Chen, Ping Yao, Dao-yong Chen. Further Expansions and Applications of the Principles and Methodology of Non-covalent Connected Micelles. [J]. Acta Polymerica Sinica 0(8):1048-1065(2018)
Guo-song Chen, Ping Yao, Dao-yong Chen. Further Expansions and Applications of the Principles and Methodology of Non-covalent Connected Micelles. [J]. Acta Polymerica Sinica 0(8):1048-1065(2018) DOI： 10.11777/j.issn1000-3304.2018.18064.
摘要
20世纪末，江明等在其有关大分子络合的研究基础上，通过将大分子间相互作用局域化，成功地利用大分子间的络合来驱动结构规整组装体的形成. 这一思想和方法通过不断地拓展和深化，形成了大分子自组装的新路线，获得了一系列具有新颖结构与功能的核壳间为非共价键连接的聚合物胶束(non-covalently connected micelles
NCCM). 本综述将对近年来我们在非共价键胶束方法与原理的拓展与应用方面取得的成果作一总结. 内容包括：为NCCM的形成引入新的驱动力，并同时赋予NCCM新的性质与功能；将NCCM 的形成原理应用于生物大分子的自组装，发展出了全绿色的大分子自组装路线；运用将相互作用局域化的基本思想，将嵌段共聚物的化学交联反应局域化，发展出化学交联诱导嵌段共聚物胶束化的新方法.
Abstract
At the end of the last century
Professor Jiang Ming
et al
. succeeded in fabricating regular nanostructures through localizing interactions in the systems of polymer complexes. Through continuous expansion and deepening of this principle and method
a new strategy of macromolecular self-assembly was established. This review summarizes recent developments and applications of non-covalently connected micelles (NCCMs)
including: Introducing of new driving forces such as supramolecular interactions to drive the formation of NCCMs
providing the resultant NCCMs with new features and functions; Applying the principle to the self-assembly of biological macromolecules
thereby developing an entirely green route to self-assembly of macromolecules; Also
through localizing covalent crosslinking reaction of one block of a diblock copolymer
we realized micellization of the block copolymer in its common solvent induced by the crosslinking reaction
resulting in highly efficient fabrication of core-stabilized micelles as well as a new pathway for controlling the kinetics of polymer micellization
the structures and the properties of the polymeric micelles.
关键词
非共价键连接胶束大分子自组装超分子相互作用非共价键生物大分子自组装
Keywords
Non-covalent connected micellesMacromolecular self-assemblySupramolecular interactionsNon-covalent bondsBiomacromolecular self-assembly
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