Double-cable Conjugated Polymers and Their Application in Single-component Organic Solar Cells

Wei-wei Li

doi:10.11777/j.issn1000-3304.2019.18212

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Double-cable Conjugated Polymers and Their Application in Single-component Organic Solar Cells

Feature Articles | 更新时间：2021-01-26

- Double-cable Conjugated Polymers and Their Application in Single-component Organic Solar Cells
- Acta Polymerica Sinica Vol. 50, Issue 3, Pages: 209-218(2019)
- 作者机构：
  
  中国科学院化学研究所　北京 100190
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2019.18212
  CLC：
- Published：2019-3，
  
  Published Online：21 November 2018，
  
  Received：10 October 2018，
  
  Revised：1 November 2018，
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Wei-wei Li. Double-cable Conjugated Polymers and Their Application in Single-component Organic Solar Cells. [J]. Acta Polymerica Sinica 50(3):209-218(2019)
DOI：

Wei-wei Li. Double-cable Conjugated Polymers and Their Application in Single-component Organic Solar Cells. [J]. Acta Polymerica Sinica 50(3):209-218(2019) DOI： 10.11777/j.issn1000-3304.2019.18212.

摘要

给体/受体型双缆共轭聚合物是一类含给体主链与受体侧链的共轭聚合物，通过分子内相分离形成异质结，从而应用于单组分有机太阳能电池中. 双缆共轭聚合物及其单组分有机太阳能电池的研究均处于初级阶段，光电转换性能远低于本体异质结太阳能电池. 本文总结了单组分有机太阳能电池的研究进展，重点介绍了我们在双缆共轭聚合物的结构设计、相分离调控以及单组分太阳能电池性能方面的研究工作，并论述了双缆共轭聚合物及其单组分有机太阳能电池存在的科学问题及发展方向.

Abstract

Bulk-heterojunction (BHJ) structures that comprise donor and acceptor blended physically in photoactive layers are proved very promising for applications in organic solar cells

of which a power conversion efficiency (PCE) of 15% has already been achieved in single-junction devices. However

their nanophase separation is susceptible to heat and light and hence lower the stability of solar cells during long-term service. To this end

single-component organic solar cells (SCOSCs) are developed as potential alternatives with better photovoltaic stability. Double-cable conjugated polymers

which consist of electron-rich conjugated backbone and electron-deficient conjugated side chains

can be applied into SCOSCs by forming BHJ structures in a single conjugated polymer. Relevant research on double-cable conjugated polymers and SCOSCs has rarely been reported in the past years and their PCEs lagged far behind those of the BHJ solar cells. Herein

we first provide a general review on the research progress of SCOSCs and then center the discussion on some recent findings in our group about double-cable conjugated polymers

including the development of new synthetic methods

the design ideas for novel double-cable polymers composed of varied conjugated backbones with conjugated side chains and linkers

the tuning approaches toward nanophase separation in double-cable polymers

and the ultimate applications in SCOSCs. Given the existing studies

we believe that SCOSCs based on double-cable polymers will receive more attention and advance further with higher PCEs in the near future.

关键词

双缆共轭聚合物有机太阳能电池单组分相分离

Keywords

Double-cable polymerOrganic solar cellSingle-componentPhase separation

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College of Chemistry and Chemical Engineering, Jiangxi University of Science and Technology

State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology

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Bohai Rim Collaborative Innovation Center on Green Chemical Application Technology, Department of Chemical Engineering, Weifang Vocational College

Department of Polymer Science and Engineering, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University

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