Synthesis and Applications of Porous Graphene

Deng Zhou; Ming Li

doi:10.11777/j.issn1000-3304.2019.19014

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Synthesis and Applications of Porous Graphene

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- Synthesis and Applications of Porous Graphene
- Acta Polymerica Sinica Vol. 50, Issue 7, Pages: 671-684(2019)
- 作者机构：
  
  有机功能分子合成与应用教育部重点实验室有机化工新材料湖北省协同创新中心高分子材料湖北省重点实验室湖北大学化学化工学院　武汉 430062
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2019.19014
  CLC：
- Published：2019-7，
  
  Published Online：9 April 2019，
  
  Received：17 January 2019，
  
  Revised：1 March 2019，
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Deng Zhou, Ming Li. Synthesis and Applications of Porous Graphene. [J]. Acta Polymerica Sinica 50(7):671-684(2019)
DOI：

Deng Zhou, Ming Li. Synthesis and Applications of Porous Graphene. [J]. Acta Polymerica Sinica 50(7):671-684(2019) DOI： 10.11777/j.issn1000-3304.2019.19014.

摘要

石墨烯由于其优异的性能，例如高比表面积、高导电性、良好的热稳定性和优异的机械强度，引起了人们极大的研究兴趣. 但是石墨烯本身不具有固有孔隙. 为了使其具有固有孔隙，各种多孔石墨烯材料被制备出来，例如，全碳型多孔石墨烯、掺杂型多孔石墨烯及多孔石墨烯复合材料等等. 由于多孔石墨烯既能保留原始石墨烯的部分性质，又比原始石墨烯具有更高的比表面积和孔隙体积，它在光电子器件、储能、气体分离/储存、废水分离及光催化等领域都具有巨大的应用前景. 本文主要回顾各种多孔石墨烯材料的合成方法以及这些材料在各个领域的应用，并展望了多孔石墨烯材料在合成和应用中的机遇和挑战.

Abstract

Graphene is an sp

carbon material having a hexagonal honeycomb lattice in a single-layer two-dimensional (2D) plane due to its excellent properties such as high specific surface area

high electrical conductivity

good thermal stability and excellent mechanical properties. It has already aroused great research interest. Porous graphene refers to a carbon material possessing nano-scale pores in a two-dimensional plane. Due to the introduction of pores

not only the accumulation caused by

electron interaction is effectively avoided

but also some properties of the original graphene can be retained for porous graphene with higher specific surface area and pore volume. And also

the band gap of graphene was effectively opened. Therefore

it has great application prospects in the fields of optoelectronic devices

energy storage

gas separation/storage

wastewater separation and photocatalysis. At present

various porous graphene materials (for example

all-carbon porous graphene

doped porous graphene

and porous graphene composite materials

etc.

) prepared by chemical synthesis

hydrothermal method

electrochemical reduction method

and template-oriented chemical vapor deposition (CVD) method

have been well applied in various fields. This paper aims to summarize the design and synthesis of various porous graphene materials

and also discusses the characteristics

advantages and disadvantages of porous graphene and various potential applications as well as the comparison of various porous graphene structures and properties. And looking forward to future research

it may focus on developing simpler

more convenient synthesis methods and how to accurately control the size

structure

and distribution density of pores in porous graphene

how to precisely control the type and distribution of doping elements

and how to better couple with other materials to obtain better composite materials

making porous graphene more excellent in various applications.

关键词

石墨烯多孔材料比表面积掺杂复合材料

Keywords

GraphenePorous materialSpecific surface areaDopingComposite

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Department of Chemistry, Tsinghua University

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Institute of Flexible Electronics (SIFE), Northwestern Polytechnical University

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