Progress of Strategies for Improving Thermoelectric Performance of Poly(3,4-ethylenedioxythiophene):Poly(styrene sulfonate)

Xuan Huang; Zhuo-xin Liu; Fu-sheng Liu; Guang-ming Chen

doi:10.11777/j.issn1000-3304.2020.20245

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Progress of Strategies for Improving Thermoelectric Performance of Poly(3,4-ethylenedioxythiophene):Poly(styrene sulfonate)

Reviews | 更新时间：2021-03-29

- Progress of Strategies for Improving Thermoelectric Performance of Poly(3,4-ethylenedioxythiophene):Poly(styrene sulfonate)
- Acta Polymerica Sinica Vol. 52, Issue 4, Pages: 339-349(2021)
- 作者机构：
  
  深圳大学材料学院　深圳 518055
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2020.20245
  CLC：
- Published：3 April 2021，
  
  Published Online：14 December 2020，
  
  Received：4 November 2020，
  
  Revised：19 November 2020，
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Xuan Huang, Zhuo-xin Liu, Fu-sheng Liu, Guang-ming Chen. Progress of Strategies for Improving Thermoelectric Performance of Poly(3,4-ethylenedioxythiophene):Poly(styrene sulfonate). [J]. Acta Polymerica Sinica 52(4):339-349(2021)
DOI：

Xuan Huang, Zhuo-xin Liu, Fu-sheng Liu, Guang-ming Chen. Progress of Strategies for Improving Thermoelectric Performance of Poly(3,4-ethylenedioxythiophene):Poly(styrene sulfonate). [J]. Acta Polymerica Sinica 52(4):339-349(2021) DOI： 10.11777/j.issn1000-3304.2020.20245.

摘要

近十年，有机聚合物及其复合热电材料与柔性器件取得了显著进展，在废热回收利用、可穿戴电子学、软体机器人和物联网等领域有广泛的应用. 其中，聚(3

4-乙烯二氧噻吩):聚苯乙烯磺酸(PEDOT:PSS)是迄今研究最多也是性能最高的聚合物体系. 本文对近年来有关PEDOT:PSS热电性能有效提升主要策略的文献报道进行了总结. 首先，从PEDOT:PSS的二次掺杂/去掺杂、酸或碱处理和离子液体处理方面等，重点论述了掺杂/去掺杂策略的研究进展；然后，分别从改善聚集态结构、构筑PEDOT微纳米结构和与碳纳米材料复合等3个方面，重点介绍了采用此3种策略提升PEDOT:PSS热电性能的研究进展；最后，对该领域进行总结，提出了开展进一步研究的建议，并对其未来发展前景进行展望.

Abstract

In the recent decade

due to their versatile advantages of solution processability

light-in-weight

super flexibility

low thermal conductivity and highly adjustable molecular structures or components

organic and organic/inorganic composite thermoelectric materials as well as their flexible devices have made great progress. A variety of judicious strategies of both material preparation and flexible device assembly have been developed to improve the corresponding thermoelectric performances. Hence

they are very promising for wide application fields

including harvesting of waste heat

flexible electronics

soft robotics and internet-of-things. So far

in all of the reported organic polymer and composite thermoelectric materials

poly(3

4-ethylene dioxyethiophene):poly(styrene sulfonate) (PEDOT:PSS) is probably the most frequently studied and most successful system with the highest thermoelectric performance. Nevertheless

compared with inorganic thermoelectric materials

the thermoelectric properties of PEDOT:PSS is distinctly lower than the maximum value of the inorganic counterparts. Considering the fact of few special reviews about the strategies to effectively enhance the thermoelectric performances for PEDOT:PSS to date

it is timely and urgent to publish a relevant review. Here

we present a summarization of the recent progress in the development of strategies to significantly enhance the thermoelectric properties of PEDOT:PSS developed so far. First

the advances of the doping/de-doping strategies

such as second doping/de-doping

acid or alkali treatment

and treating by ionic liquid

are focused in details. The corresponding mechanism is discussed as well. Then

the recent developments of three types of boosting strategies

i.e.

tuning of aggregation structures (including crystalline and orientation microstructures)

construction of PEDOT nano-micro structures (for example

nanospheres

nanorods

micro- or nano-tubes and nanofibers)

and fabrication of thermoelectric composites with inorganic particles such as carbon nanotubes and graphene nanoplatelets

are concentrated. The relevant thermoelectric properties are compared. Finally

we conclude that some strategies to effectively enhance the thermoelectric properties for PEDOT:PSS have been successfully developed

and there is still a long way to go for the actual applications. In particular

three tentative suggestions to the future investigations are proposed

i.e.

in-depth investigation of the mechanism between microstructure and thermoelectric performances for the neat PEDOT:PSS

developing novel fabrication procedures with strong interfacial interaction like covalent-bonding and the relevant mechanism study

and exploiting of precise measurement techniques for the thermoelectric parameters of films

hydrogels and aerogels. Finally

the prospects of the future work are outlooked.

关键词

聚(34-乙烯二氧噻吩):聚(苯乙烯磺酸)热电性能结构-性能关系

Keywords

Poly(34-ethylenedioxythiophene):poly(styrene sulfonate)Thermoelectric propertiesStructure-performance relationship

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