Insulating Polymer Additives for Improving the Efficiency and Stability of Organic Solar Cells

Lang-kun Chen; Sheng-hua Liu

doi:10.11777/j.issn1000-3304.2021.21120

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Insulating Polymer Additives for Improving the Efficiency and Stability of Organic Solar Cells

Reviews | 更新时间：2022-07-08

- Insulating Polymer Additives for Improving the Efficiency and Stability of Organic Solar Cells
- ACTA POLYMERICA SINICA Vol. 52, Issue 11, Pages: 1459-1472(2021)
- 作者机构：
  
  中山大学材料学院深圳 518107
- 作者简介：
- 基金信息：
- DOI：10.11777/j.issn1000-3304.2021.21120
  CLC：
- Published：20 November 2021，
  
  Published Online：22 July 2021，
  
  Received：25 April 2021，
  
  Revised：20 May 2021，
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陈朗昆,刘升华.绝缘聚合物添加剂：提高有机太阳能电池的效率及稳定性[J].高分子学报,2021,52(11):1459-1472.

Chen Lang-kun,Liu Sheng-hua.Insulating Polymer Additives for Improving the Efficiency and Stability of Organic Solar Cells[J].ACTA POLYMERICA SINICA,2021,52(11):1459-1472.
陈朗昆,刘升华.绝缘聚合物添加剂：提高有机太阳能电池的效率及稳定性[J].高分子学报,2021,52(11):1459-1472. DOI： 10.11777/j.issn1000-3304.2021.21120.

Chen Lang-kun,Liu Sheng-hua.Insulating Polymer Additives for Improving the Efficiency and Stability of Organic Solar Cells[J].ACTA POLYMERICA SINICA,2021,52(11):1459-1472. DOI： 10.11777/j.issn1000-3304.2021.21120.

摘要

近年来，随着活性层给体和受体材料的发展，单结有机太阳能电池(OSCs)的器件效率已经突破18%，被视为具有广阔应用前景的第三代光伏器件之一. 但OSCs的稳定性偏低一直是阻碍其产业化应用的最大瓶颈，且实现器件效率和稳定性的同步提升仍面临不小的挑战. 其中一个行之有效的策略是在OSCs中引入不同类型的添加剂. 本文总结了OSCs在提升器件效率和稳定性方面的挑战，综述了近年来一系列绝缘聚合物作为活性层添加剂在OSCs中应用的研究进展，从绝缘聚合物与活性层给体、受体材料形成三元共混结构和自组装迁移形成界面层两方面论述了提高器件效率和稳定性的方法. 最后指出了绝缘聚合物作为光伏器件添加剂的发展潜力和应用前景.

Abstract

In recent years

with the development of donors and acceptors in active layer

the efficiency of single-junction organic solar cells (OSCs) has now exceeded 18%

which is regarded as one of the third-generation photovoltaics with broad application prospects. However

the relatively low stability of the devices remains the biggest bottleneck

which hinders the industrial application of the OSCs. And the simultaneous improvement of the device efficiency and stability still faces a big challenge. One of the effective strategies is to introduce various types of additives into the OSCs. As one of the most potential additives in OSCs

insulating polymers are capable of forming ternary hybrid structures with donors and acceptors

or have good self-assembly properties

which improve the PCE effectively. Meanwhile

due to their excellent stability or physical properties

insulating polymers are conducive to maintaining the morphology of the active layer and isolating oxygen and water

which enhance the stability of devices and greatly promote the development of OSCs. The challenges of device efficiency and stability that OSCs faces are summarized. The recent research progress of a series of insulating polymers as active layer additives in the applications of OSCs is reviewed. The methods for improving the efficiency and stability of devices in terms of the formation of ternary blend structures between the insulating polymers and active layer materials

as well as the formation of interface structures by self-assembly and migration are systematically discussed. Finally

the potential and application prospects of insulating polymers as additives in photovoltaic devices are indicated.

关键词

有机太阳能电池绝缘聚合物自组装玻璃化温度界面层

Keywords

Organic solar cellsInsulating polymersSelf-assemblyGlass transition temperatureInterface layer

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苏州市新型半导体光电材料与器件重点实验室苏州大学

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State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology

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