非富勒烯聚合物太阳电池研究进展

宾海军; 李永舫

doi:10.11777/j.issn1000-3304.2017.17119

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非富勒烯聚合物太阳电池研究进展

综述 | 更新时间：2021-01-27

- 非富勒烯聚合物太阳电池研究进展
- Recent Research Progress of Photovoltaic Materials for Nonfullerene Polymer Solar Cells
- 高分子学报 2017年第9期页码：1444-1461
- 作者机构：
  
  1.中国科学院科教融合分子科学卓越中心中国科学院化学研究所有机固体院重点实验室北京 100190
  2.中国科学院大学化学化工学院北京 10004
  3.苏州大学材料与化学化工学部先进光电材料实验室苏州 215123
- 作者简介：
  
  李永舫, E-mail:liyf@iccas.ac.cn Yong-fang Li, E-mail:liyf@iccas.ac.cn
- 基金信息：
  
  国家自然科学基金(91633301);国家自然科学基金(91333204);中国科学院B类先导专项(XDB12030200);国家重点基础研究发展计划(973计划);国家自然科学基金(91433117);国家重点基础研究发展计划(2014CB643501)
- DOI：10.11777/j.issn1000-3304.2017.17119
  中图分类号：
- 纸质出版日期：2017-9，
  
  收稿日期：2017-5-2，
  
  修回日期：2017-6-26，
扫描看全文
宾海军, 李永舫. 非富勒烯聚合物太阳电池研究进展[J]. 高分子学报, 2017,(9):1444-1461.

Bin Hai-jun, Li Yong-fang. Recent Research Progress of Photovoltaic Materials for Nonfullerene Polymer Solar Cells[J]. Acta Polymerica Sinica, 2017,(9):1444-1461.
宾海军, 李永舫. 非富勒烯聚合物太阳电池研究进展[J]. 高分子学报, 2017,(9):1444-1461. DOI： 10.11777/j.issn1000-3304.2017.17119.

Bin Hai-jun, Li Yong-fang. Recent Research Progress of Photovoltaic Materials for Nonfullerene Polymer Solar Cells[J]. Acta Polymerica Sinica, 2017,(9):1444-1461. DOI： 10.11777/j.issn1000-3304.2017.17119.

摘要

综述了以

-型共轭聚合物为给体、

-型有机半导体为受体的非富勒烯聚合物太阳电池光伏材料最新研究进展，包括

-型共轭聚合物和可溶液加工小分子

-型有机半导体（

-OS）受体光伏材料，以及与之匹配的

-型共轭聚合物给体光伏材料.介绍的

-型共轭聚合物受体光伏材料包括基于苝酰亚胺（BDI）、萘酰亚胺（NDI）以及新型硼氮键连受体单元的D-A共聚物受体光伏材料，目前基于聚合物给体（J51）和聚合物受体（N2200）的全聚合物太阳电池的能量转换效率最高达到8.26%.

-OS小分子受体光伏材料包括基于BDI和NDI单元的有机分子、基于稠环中心给体单元的A-D-A型窄带隙有机小分子受体材料等.给体光伏材料包括基于齐聚噻吩和苯并二噻吩（BDT）给体单元的D-A共聚物，重点介绍与窄带隙A-D-A结构小分子受体吸收互补的、基于噻吩取代BDT单元的中间带隙二维共轭聚合物给体光伏材料.使用中间带隙的

-型共轭聚合物为给体、窄带隙A-D-A结构有机小分子为受体的非富勒烯聚合物太阳电池能量转换效率已经突破12%，展示了光明的前景.最后对非富勒烯聚合物太阳电池将来的发展进行了展望.

Abstract

Nonfullerene polymer solar cells (PSCs) based on

-type conjugated polymer as donor and

-type organic semiconductor (

-OS) as acceptor have attracted great attention in recent years

due to the advantages of the

-OS acceptors

such as strong and broad absorption in visible-NIR region

easy tuning of absorption and electronic energy levels

and good morphology stability in comparison with the traditional fullerene derivative acceptors. This article reviews the recent research progress of the

-OS acceptors (including

-type conjugated polymers and

-OS solutio

-processable organic small molecules) and the conjugated polymer donor photovoltaic materials for the application in nonfullerene PSCs. The

-type conjugated polymer acceptor materials include the perylene diimide (PDI)-and naphthalene diimide (NDI)-based D-A copolymers

as well as the D-A copolymers based on the new B←N bonded acceptor unit. The highest power conversion efficiency (PCE) reached 8.24% for the all polymer PSCs with a medium bandgap

-type conjugated polymer J51 as donor and a narrow bandgap

-type NDI-based D-A copolymer N2200 as acceptor. The

-OS small molecules acceptors include the PDI-or NDI-based molecules

the narrow bandgap A-D-A structured small molecules with a fused ring central donor unit and two electro

-withdrawing end groups (such as ITIC)

and other

-OS small molecules. The

-type conjugated polymer donor materials

matching with the nonfullerene acceptors

include the narrow bandgap oligothiophene-or banzodithiophene (BDT)-based copolymers

and the medium bandgap two-dimensio

-conjugated D-A copolymers based on BDT with thiophene conjugated side chains. The best nonfellerene PSCs

with a medium bandgap polymer as donor and a narrow bandgap A-D-A structured

-OS as acceptor

have been recently demonstrated to have high PCE of over 12%. The complementary absorption in the visible-NIR region

matching electronic energy levels of the donor and acceptor materials

is very important for the high performance nonfullerene PSCs. In the end of the article

we give some comments and point out the key issues for the next-step studies and future development of the nonfullerene PSCs.

关键词

聚合物太阳电池n-型有机半导体非富勒烯受体共轭聚合物给体光伏材料能量转换效率

Keywords

Polymer solar cellsn-type organic semiconductorsNonfullerene acceptorsConjugated polymers donor materialsPower conversion efficiency

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