共轭高分子光电功能材料的多尺度性能研究——聚合物电子学领域中的新机遇

董焕丽; 燕青青; 胡文平

doi:10.11777/j.issn1000-3304.2017.17127

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共轭高分子光电功能材料的多尺度性能研究——聚合物电子学领域中的新机遇

专论 | 更新时间：2021-01-26

- 共轭高分子光电功能材料的多尺度性能研究——聚合物电子学领域中的新机遇
- Multilevel Investigation of Charge Transport in Conjugated Polymers——New Opportunities in Polymer Electronics
- 高分子学报 2017年第8期页码：1246-1260
- 作者机构：
  
  1.中国科学院化学研究所有机固体院重点实验室北京 100190
  2.天津大学理学院天津市分子光电科学重点实验室天津大学协同创新中心天津 300072
- 作者简介：
  
  [ "董焕丽, 女, 1980年9月生.2009年于中国科学院化学研究所获得博士学位后直接留所工作至今, 先后为助理研究员、副研究员和研究员.主要研究方向为有机高分子光电功能材料与器件, 包括共轭高分子材料体系的本征性能研究和新型光电集成有机高分子功能材料设计合成及器件应用" ]
- 基金信息：
  
  国家自然科学基金(91433115);国家自然科学基金(51222306)
- DOI：10.11777/j.issn1000-3304.2017.17127
  中图分类号：
- 纸质出版日期：2017-8，
  
  收稿日期：2017-5-11，
  
  修回日期：2017-5-15，
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董焕丽, 燕青青, 胡文平. 共轭高分子光电功能材料的多尺度性能研究——聚合物电子学领域中的新机遇[J]. 高分子学报, 2017,(8):1246-1260.

Dong Huan-li, Yan Qing-qing, Hu Wen-ping. Multilevel Investigation of Charge Transport in Conjugated Polymers——New Opportunities in Polymer Electronics[J]. Acta Polymerica Sinica, 2017,(8):1246-1260.
董焕丽, 燕青青, 胡文平. 共轭高分子光电功能材料的多尺度性能研究——聚合物电子学领域中的新机遇[J]. 高分子学报, 2017,(8):1246-1260. DOI： 10.11777/j.issn1000-3304.2017.17127.

Dong Huan-li, Yan Qing-qing, Hu Wen-ping. Multilevel Investigation of Charge Transport in Conjugated Polymers——New Opportunities in Polymer Electronics[J]. Acta Polymerica Sinica, 2017,(8):1246-1260. DOI： 10.11777/j.issn1000-3304.2017.17127.

摘要

共轭高分子材料特异的金属或半导体的电子特性兼有质轻、价廉、易于加工的优点使其在有机场效应晶体管、有机太阳能电池和有机发光二极管等领域显示了重要的应用前景.然而，尽管经过几十年的不断研究，共轭高分子材料种类及其相关器件性能均已得到显著发展，但是共轭高分子材料的本征电荷传输特性仍不清楚，其研究面临巨大挑战，这主要是由共轭高分子材料本身分子量分布弥散、分子间相互缠结以及在常规旋涂薄膜器件中分子高度无序等特性所决定的.从调控共轭高分子聚集态结构的角度出发，不断提高共轭高分子的结构有序性及减小电荷传输过程中的晶界及缺陷密度，是实现共轭高分子材料本征性能认识的有效途径之一.本文首先简单归纳总结了研究者在共轭高分子多尺度聚集态结构调控及性能研究方面的初步结果，进一步结合国内外相关研究进展，重点对共轭高分子晶体方面的工作展开详细介绍，最后对该领域未来发展的挑战及机遇进行了简单评述.

Abstract

Conjugated polymers have demonstrated promising applications in fields of organic field-effect transistors

organic solar cells and organic light-emitting diodes

etc

due to their attractive advantages of unique optoelectronic properties

light weight

low cost and easy processability. However

regardless of the remarkable development for conjugated polymer materials and devices over the past decades

charge transport in conjugated polymers still remains unclear

which is mainly due to the molecular weight polydispersity and intermolecular entanglements of conjugated polymers as well as their naturally disordered structures in films. To achieve better understanding of the nature charge transport in conjugated polymers

continually increasing the molecular orders and reducing grain boundaries and defects are crucial. Aiming at this point

we propose a concept of multilevel charge transport investigation in conjugated polymers

and under this guideline

we have carried out systematical studies over the past years. In this article

we briefly summarize our recent results on charge transport investigation in conjugated polymers from macro-

to micro/nano-and molecular scales. With a derivative of poly(paraphenylene ethynylene) with thioacetyl end groups (TA-PPE) selected as an example

we found that the charge transport property could be significantly improved by 3-4 orders by continuously increasing the molecular orders in solid state. With downscaling to molecular scale

some new phenomenon was observed for conjugated polymers

such as the modulation of the redox center of tetrathiafulvalene (TTF) units on tunneling charge transport. In part 2 of the paper

combining the recent progress in literature

we give a detailed demonstration on the development history of conjugated polymer single crystals

with special emphasis on our efforts carried out in this field. Based on the investigation of polymer single crystals

a novel molecular packing model is found in the polymer micro/nanowires

that is the conjugated polymers aligned along the long-axis of nanowires

and the investigation of intrachain and interchain charge transport is achieved based on an individual conjugated polymer crystal

which is an important step in this filed. Finally

a short outlook is provided with regard to the concerns and the opportunities for the future studies on the multilevel properties and the devices of the conjugated polymers.

关键词

共轭高分子材料多尺度聚集态结构共轭高分子晶体本征性能高性能器件

Keywords

Conjugated polymersMultilevel solid state structuresConjugated polymer single crystalsIntrinsic propertyHigh performance devices

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