高分子发光材料研究进展

邵世洋; 丁军桥; 王利祥

doi:10.11777/j.issn1000-3304.2018.17289

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高分子发光材料研究进展

专论 | 更新时间：2021-01-26

- 高分子发光材料研究进展
- Research Progress on Electroluminescent Polymers
- 高分子学报 2018年第2期页码：198-216
- 作者机构：
  
  中国科学院长春应用化学研究所高分子物理与化学国家重点实验室长春 130022
- 作者简介：
  
  丁军桥, E-mail: junqiaod@ciac.ac.cn Jun-qiao Ding, E-mail: junqiaod@ciac.ac.cn
  王利祥, E-mail: lixiang@ciac.ac.cn Li-xiang Wang, E-mail: lixiang@ciac.ac.cn
- 基金信息：
  
  国家自然科学基金(51573182);国家自然科学基金(51203149);国家自然科学基金(91333205);国家重点基础研究发展计划(973计划)(2015CB655000)
- DOI：10.11777/j.issn1000-3304.2018.17289
  中图分类号：
- 纸质出版日期：2018-2-20，
  
  收稿日期：2017-10-17，
  
  修回日期：2017-11-3，
扫描看全文
邵世洋, 丁军桥, 王利祥. 高分子发光材料研究进展[J]. 高分子学报, 2018,(2):198-216.

Shao Shi-yang, Ding Jun-qiao, Wang Li-xiang. Research Progress on Electroluminescent Polymers[J]. Acta Polymerica Sinica, 2018,(2):198-216.
邵世洋, 丁军桥, 王利祥. 高分子发光材料研究进展[J]. 高分子学报, 2018,(2):198-216. DOI： 10.11777/j.issn1000-3304.2018.17289.

Shao Shi-yang, Ding Jun-qiao, Wang Li-xiang. Research Progress on Electroluminescent Polymers[J]. Acta Polymerica Sinica, 2018,(2):198-216. DOI： 10.11777/j.issn1000-3304.2018.17289.

摘要

高分子发光材料具有可溶液加工的特点，适于制备低成本、大面积发光器件，在平板显示和固体照明领域具有潜在的应用前景.近年来，高分子发光材料在发光机制、材料体系和器件性能等方面均取得了重要进展，各项性能得到了大幅度提升.本文从材料和器件角度，围绕高分子荧光材料、高分子磷光材料和高分子热活化延迟荧光材料的分子设计策略，总结和评述了高分子荧光材料的颜色调控和效率提升途径，高分子磷光材料的磷光掺杂剂、高分子主体、拓扑结构等因素对发光性能的影响规律，以及高分子热活化延迟荧光材料的设计原理和典型材料体系.同时，分析了高分子发光材料未来发展面临的机遇和挑战.

Abstract

Electroluminescent polymers hold great promise in penal display and solid-state lighting applications because of their advantages of solution processability

large-scale manufacturing and ability to produce flexible devices based on plastic substrates. In the past decades

great progress has been made in electroluminescent polymers including their working mechanism

material systems and device performance. Basically

electroluminescent polymers can be divided into three classes:fluorescent polymers

phosphorescent polymers and thermally activated delayed fluorescence (TADF) polymers. For fluorescent polymers

the internal quantum efficiency (IQE) is limited to 25% because they can use only singlet excitons in the electroluminescent device. In comparison

IQE of phosphorescent polymers can reach 100% because of the strong spin-orbital coupling induced by the heavy-atoms in the phosphorescent dopants. Recently

TADF polymers have evolved rapidly as the new kind of electroluminescent polymers because they are able to utilize triplet excitons through rapid reverse intersystem crossing process from the lowest triplet state to the lowest singlet state

thereby providing a promising approach to reach 100% IQE without the use of noble metal elements. With these developments

the device performance of the polymers has been enhanced greatly and many indexes have met the commercialization requirements. This review is aimed to summarize the research progresses on electroluminescent polymers used for organic light-emitting diodes

including the molecular design and device performance of representative examples of fluorescent polymers

phosphorescent polymers and TADF polymers. The emphasis of this review is especially focused on the color tuning and performance improvement approaches for the fluorescent polymers

the optimization of the phosphorescent dopant

the polymer host and the topological structure of the phosphorescent polymers

as well as the design principles of the thermally activated delayed fluorescence polymers. Finally

the perspectives and the key challenges of the electroluminescent polymers are discussed

and future directions of efforts toward further developing low-cost

efficient

and stable electroluminescent polymers are also demonstrated.

关键词

高分子发光材料高分子荧光材料高分子磷光材料高分子热活化延迟荧光材料

Keywords

Electroluminescent polymerFluorescent polymerPhosphorescent polymerThermally activated delayed fluorescence polymer

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