可持续高分子-纤维素新材料研究进展

段博; 涂虎; 张俐娜

doi:10.11777/j.issn1000-3304.2020.19160

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可持续高分子-纤维素新材料研究进展

综述 | 更新时间：2021-04-27

- 可持续高分子-纤维素新材料研究进展
- Material Research Progress of the Sustainable Polymer-Cellulose
- 高分子学报 2020年51卷第1期页码：66-86
- 作者机构：
  
  武汉大学化学与分子科学学院　武汉 430072
- 作者简介：
  
  [ "段博，男，1987年生，副研究员. 2015年毕业于武汉大学化学与分子科学学院并获得理学博士学位. 2016 ~ 2019年在美国斯托瓦斯研究所从事博士后工作，研究生殖干细胞分化微环境. 2019年6月进入武汉大学化学与分子科学学院从事天然高分子方面的研究工作. 主要研究方向为甲壳素、纤维素功能材料的开发" ]
  [ "张俐娜，女，1940年生，教授/博导，中国科学院院士. 1963年毕业于武汉大学化学系. 1985年曾获日本政府学术振兴协会奖学金(JSPS)赴大阪大学研究近2年. 1993年创立天然高分子科研组，2011年当选中国科学院院士，2014年为英国皇家化学会会士. 现任美国化学会刊物ACS Sustainable Chemistry & Engineering的副主编以及多家国内外刊物编委. 基础研究成果已在国内外刊物发表论文600余篇，其中560余篇发表在国际SCI源刊上，被他人引用近18000次；主编专著15部；获准专利100余项；荣获国家自然科学奖二等奖1项，省级自然科学一等奖1项及技术发明一等奖1项；获美国化学会2011年Anselme Payen奖(国际纤维素与可再生资源材料领域最高奖). 曾获全国优秀教师和全国先进工作者等国家级荣誉. 主要研究方向为高分子物理、天然高分子改性材料、复杂多糖的分子和链构象与其生物活性关系" ]
- 基金信息：
  
  国家自然科学基金重大项目(基金号 21334005)资助
- DOI：10.11777/j.issn1000-3304.2020.19160
  中图分类号：
- 纸质出版日期：2020-1，
  
  网络出版日期：2019-11-19，
  
  收稿日期：2019-8-30，
  
  修回日期：2019-9-27，
扫描看全文
段博, 涂虎, 张俐娜. 可持续高分子-纤维素新材料研究进展[J]. 高分子学报, 2020,51(1):66-86.

Bo Duan, Hu Tu, Li-na Zhang. Material Research Progress of the Sustainable Polymer-Cellulose[J]. Acta Polymerica Sinica, 2020,51(1):66-86.
段博, 涂虎, 张俐娜. 可持续高分子-纤维素新材料研究进展[J]. 高分子学报, 2020,51(1):66-86. DOI： 10.11777/j.issn1000-3304.2020.19160.

Bo Duan, Hu Tu, Li-na Zhang. Material Research Progress of the Sustainable Polymer-Cellulose[J]. Acta Polymerica Sinica, 2020,51(1):66-86. DOI： 10.11777/j.issn1000-3304.2020.19160.

摘要

21世纪“绿色”化学已成为世界各国社会经济发展中的研究与开发战略方向. 纤维素是自然界中储量最丰富的天然高分子，是重要的可再生资源以及未来的主要工业原料. 然而由于纤维素存在着大量的分子内以及分子间氢键，其结构致密，难以溶解或熔融进一步加工. 本文简要介绍了近几年来关于直接使用物理溶剂方法(非衍生化)对纤维素材料开发利用的新进展，主要包括以下4个方面：(1)纤维素在“绿色”溶剂-碱/尿素以及离子液体体系中的溶解和再生；(2)纳米纤维素的制备以及组装；(3)木材纳米技术的开发及利用；(4)细菌纤维素基材料等，旨在推进“绿色”技术实现纤维素资源的研究开发及利用.

Abstract

The “Green Chemistry” has become the strategy direction of research and development of the world in the 21

century. Cellulose

as the most abundant natural polymers

is a very important renewable resource and the main industrial raw material. The cellulose shows many great advances including biocompatibility

biodegradability

high structure stability. However

due to the large amounts of inter- and intra-hydrogen bonding among the cellulose molecules

the cellulose has a dense structure and is very hard to be processed through dissolution or melt

which limit the further exploitation of the cellulose resource. The traditional organic solution of the cellulose often has the problem of high cost and pollution. In recent decades

with the development of the “Green” solvent (alkaline/urea

ionic liquid

etc

.) and the cellulose nanotechnology

the researchers have greatly expanded the cellulose application in biomedical

energy storage

optical fields in addition to the traditional spinning and papermaking industry. This review mainly introduces the new methods (“bottom to up” and “up to down”) for the exploitation of cellulose based materials in recent years through the following four sections: (1) the regenerated cellulose based materials from the “green” solution-alkaline/urea aqueous and ionic liquid; (2) the preparation and self-assembly of the nanocellulose; (3) the development and utilization of the wood nanotechnology; (4) bacterial cellulose based functional materials.

关键词

纤维素可持续高分子碱/尿素离子液体纳米纤维素纳米技术细菌纤维素

Keywords

“Green” chemistryAlkaline/UreaIonic liquidNanocelluloseWood nanotechnologyBacterial cellulose

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