高分子材料图案记忆表面

陈帅; 严淑珍; 印杰; 姜学松

doi:10.11777/j.issn1000-3304.2021.21072

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高分子材料图案记忆表面

专论 | 更新时间：2023-12-20

- 高分子材料图案记忆表面
- Pattern Memory Surface (PMS) of Polymer
- 高分子学报 2021年52卷第10期页码：1245-1261
- 作者机构：
  
  上海交通大学化学化工学院金属基复合材料国家重点实验室变革性分子前沿科学中心上海 200240
- 作者简介：
  
  [ "姜学松，男，1977年生. 上海交通大学化学化工学院研究员，博导生导师. 2005年于上海交通大学获得博士学位，同年任教于上海交通大学，2014年晋升为研究员. 2009~2010年在德国哥廷根大学进行洪堡博士后研究，2012年入选教育部“新世纪优秀人才”，2015和2020年分别获得国家自然科学优秀青年基金和杰出青年基金. 研究方向为智能高分子材料及其表面图案，发展了构建动态微纳米褶皱图案的新策略，实现了表面褶皱的二维严格有序. 近年来在《Natl Sci Rev》《Acc Chem Res》《Sci Adv》《Nat Commun》《Adv Mater》《Angew Chem》等期刊上发表论文110余篇，授权国内外专利20多项." ]
- 基金信息：
  
  国家自然科学基金(基金号 ┣52025032);51773114┫
- DOI：10.11777/j.issn1000-3304.2021.21072
  中图分类号：
- 纸质出版日期：2021-10-20，
  
  网络出版日期：2021-08-18，
  
  收稿日期：2021-03-09，
  
  修回日期：2021-04-05，
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陈帅,严淑珍,印杰等.高分子材料图案记忆表面[J].高分子学报,2021,52(10):1245-1261.

Chen Shuai,Yan Shu-zhen,Yin Jie,et al.Pattern Memory Surface (PMS) of Polymer[J].ACTA POLYMERICA SINICA,2021,52(10):1245-1261.
陈帅,严淑珍,印杰等.高分子材料图案记忆表面[J].高分子学报,2021,52(10):1245-1261. DOI： 10.11777/j.issn1000-3304.2021.21072.

Chen Shuai,Yan Shu-zhen,Yin Jie,et al.Pattern Memory Surface (PMS) of Polymer[J].ACTA POLYMERICA SINICA,2021,52(10):1245-1261. DOI： 10.11777/j.issn1000-3304.2021.21072.

摘要

微纳米图案赋予了材料表面独特的光学、电学、声学、力学以及生物学等特性，其中具有动态变化形貌的表面图案能够实现对材料表面性能原位实时调控，可用于构建智能表面. 能够改变临时拓扑形貌并在外界刺激下恢复初始状态的一类动态表面材料称为图案记忆表面(pattern memory surface

PMS). PMS在浸润性调节、智能显示、电子器件和信息安全等多个领域具有重要的应用前景，涉及化学、物理、材料和生物多个学科交叉领域，是智能材料研究热点之一. 然而，由于基底材料对高分子链在微观尺度上的运动具有束缚作用，如何构筑动态可调的拓扑形貌记忆表面一直是该领域面临的难题. 基于此，本专论试图定义高分子材料图案记忆表面特征，并总结PMS有关研究的新进展. 重点讨论基于褶皱图案构建PMS的优势，进而介绍了PMS作为智能材料在动态光栅、防伪、反射式显示、细胞培养等领域的应用，同时展望PMS的发展前景.

Abstract

Micro-Nano patterns endow material surfaces with unique optical

electrical

acoustic

mechanical and biological properties. Especially

the patterns with dynamically switchable topography can

in situ

tune the performance of surfaces on-demand and provide a promising alternative for constructing smart materials. Here

the dynamic patterned surfaces whose morphology are temporarily switchable and can return to their original states after undergoing external stimulation are classified as pattern memory surface (PMS). PMS is of great significance to chemistry

physics

materials and biology

and plays an important role in many advanced applications

such as switchable wetting

smart display

electron devices and information security. However

establishing PMS with dynamically tunable topography is still extensively challenging due to the restricted movement of polymer chains caused by substrate material. In this feature article

we attempt to define the characteristics of PMS and summarize the recent developments of the presented PMS of polymer. The strategies for fabricating PMS based on bilayer wrinkled system are emphatically discussed. In addition to the potential of promoting the next generation of smart materials

PMS holds promise in a wide range of intriguing fields as well

including dynamic grating

anti-counterfeiting

reflective display

and cell culture.

关键词

图案记忆表面动态图案褶皱刺激响应智能材料

Keywords

Pattern memory surfaceDynamic patterningWrinkled surfaceStimuli-responsive surfaceSmart materials

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