协同的共价-超分子聚合物

张照明; 赵骏; 颜徐州

doi:10.11777/j.issn1000-3304.2022.22049

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协同的共价-超分子聚合物

专论 | 更新时间：2024-10-08

- 协同的共价-超分子聚合物
- Synergistic Covalent-and-Supramolecular Polymers
- 高分子学报 2022年53卷第7期页码：691-706
- 作者机构：
  
  上海交通大学化学化工学院上海 200240
- 作者简介：
  
  [ "颜徐州，男，1986年生. 上海交通大学化学化工学院研究员，博士生导师. 2009年获得浙江理工大学学士学位，2014年获得浙江大学博士学位. 2014~2018年分别在美国犹他大学和斯坦福大学从事博士后研究工作. 2018年9月入职上海交通大学开展独立研究工作. 2018年入选上海市高校特聘教授(东方学者)支持计划，2021年获得国家自然科学基金优秀青年科学基金资助. 主要研究方向为动态高分子材料和机械互锁聚合物." ]
- 基金信息：
  
  国家自然科学基金(基金号 ┣22122105;22071152);22101175┫
- DOI：10.11777/j.issn1000-3304.2022.22049
  中图分类号：
- 纸质出版日期：2022-07-20，
  
  网络出版日期：2022-05-13，
  
  收稿日期：2022-02-23，
  
  录用日期：2022-03-24
- 稿件说明：
移动端阅览
张照明,赵骏,颜徐州.协同的共价-超分子聚合物[J].高分子学报,2022,53(07):691-706.

Zhang Zhao-ming,Zhao Jun,Yan Xu-zhou.Synergistic Covalent-and-Supramolecular Polymers[J].ACTA POLYMERICA SINICA,2022,53(07):691-706.
张照明,赵骏,颜徐州.协同的共价-超分子聚合物[J].高分子学报,2022,53(07):691-706. DOI： 10.11777/j.issn1000-3304.2022.22049.

Zhang Zhao-ming,Zhao Jun,Yan Xu-zhou.Synergistic Covalent-and-Supramolecular Polymers[J].ACTA POLYMERICA SINICA,2022,53(07):691-706. DOI： 10.11777/j.issn1000-3304.2022.22049.

摘要

共价聚合物性质稳定但缺乏动态性，超分子聚合物动态性有余而机械性能不足. 受生命体中超分子聚合物工作机制的启发，我们将共价聚合物和超分子聚合物整合到同一体系，并采用有效的连接方式将两者关联，进而融合甚至放大2种聚合物的性能优势，发展了协同的共价-超分子聚合物. 本文从协同的共价-超分子聚合物的概念及特点出发，介绍了这一特殊形式的聚合物. 然后，总结了现有的用于构筑协同的共价-超分子聚合物的聚合策略. 进一步地，重点介绍了协同聚合物的结构和性能表现，阐明协同聚合物的性能优势和构效关系. 最后，指出了协同聚合物未来发展所面临的关键问题和重要挑战. 协同的共价-超分子聚合物体系的提出，可用于克服单一聚合物体系存在的固有缺陷，推动实现超分子聚合物的现实应用，也为发展机械性能和动态性俱佳的智能高分子材料提供新思路.

Abstract

Covalent polymers are robust but not adaptive

while supramolecular polymers have fantastic dynamic properties but lack good mechanical properties

which limit their applications in specific fields. Inspired by the working mechanism of the supramolecular polymers in living organisms

covalent polymers and supramolecular polymers are integrated into one system and connect with each other by effective interactions to afford a new fashion of polymeric system named as synergistic covalent-and-supramolecular polymers (CSPs)

which can combine and even amplify the merits of the two kinds of polymers. This article first introduces the definition and features of CSPs. Then we summarize the current synthetic strategies for the synergistic CSPs. Further

the structures and properties of synergistic CSPs are emphasized to establish their relationships and elucidate property advantages of synergistic CSPs. Finally

the key scientific issues and challenges in the field of synergistic CSPs are discussed. Synergistic CSPs are beneficial to remedy the deficiencies of individual polymer

and thus prompt the practical applications of supramolecular polymers. Furthermore

it also provides a new approach to preparing polymeric materials with mechanically robust yet dynamic properties.

关键词

协同效应超分子聚合物非共价键机械性能动态材料

Keywords

Synergistic effectSupramolecular polymersNon-covalent interactionsMechanical propertiesDynamic materials

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