编织聚合物

王泽钜; 绳新如; 李光锋; 颜徐州; 黄飞鹤

doi:10.11777/j.issn1000-3304.2022.22130

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编织聚合物

综述 | 更新时间：2024-10-08

- 编织聚合物
- Woven Polymers
- 高分子学报 2022年53卷第11期页码：1301-1315
- 作者机构：
  
  1.浙江大学化学系杭州 310027
  2.浙江大学杭州国际科创中心杭州 311200
  3.上海交通大学化学化工学院上海 200240
- 作者简介：
  
  [ "李光锋，男，1989年生. 浙江大学杭州国际科创中心研究员，2018年获得复旦大学理学博士学位，2018~2021年在上海交通大学从事博士后研究工作. 2021年6月加入浙江大学杭州国际科创中心超分子新物质创制创新工坊黄飞鹤教授课题组从事研究工作. 主要研究方向为超分子聚合物和机械互锁分子材料." ]
  [ "颜徐州，男，1986年生. 上海交通大学化学化工学院研究员，博士生导师. 2009年获得浙江理工大学学士学位，2014年获得浙江大学博士学位，2014~2018年分别在美国犹他大学和斯坦福大学从事博士后研究工作. 2018年9月入职上海交通大学开展独立研究工作. 2018年入选上海市高校特聘教授(东方学者)支持计划，2021年获得国家自然科学基金优秀青年科学基金资助. 主要研究方向为动态高分子材料和机械互锁聚合物." ]
  [ "黄飞鹤，男，1973年生. 浙江大学化学系教授、浙江大学理学部副主任、浙江大学杭州国际科创中心超分子新物质创制创新工坊执行院长. 1996年获合肥工业大学学士学位. 1999年获中国科学技术大学高分子化学与物理硕士学位. 2005年获Virginia Polytechnic Institute & State University有机与高分子化学博士学位. 曾获国家杰出青年科学基金资助、中国化学会-阿克苏诺贝尔化学奖、德国Bruno Werdelmann Lectureship Award、英国皇家化学会Cram Lehn Pedersen Prize in Supramolecular Chemistry、英国皇家化学会Polymer Chemistry Lectureship Award、浙江省自然科学奖一等奖(第一完成人). 入选长江学者特聘教授、国家万人计划领军人才. 任国务院学位委员会学科评议组成员、中国化学会超分子化学专业委员会副主任委员、浙江大学新物质创制会聚研究计划首席科学家. 已发论文352篇. 论文被引33041次，H-index为99. 主要研究方向为超分子聚合物、非多孔自适应晶体(简称：纳客；英文全称：nonporous adaptive crystals；英文简称：NACs)." ]
- 基金信息：
  
  国家重点研发计划(2021YFA0910100);国家自然科学基金(基金号 ┣22035006);22122105┫;浙江省自然科学基金(基金号 LD21B020001);浙江大学上海高等研究院繁星科学基金(基金号 SN-ZJU-SIAS-006)资助项目
- DOI：10.11777/j.issn1000-3304.2022.22130
  中图分类号：
- 纸质出版日期：2022-11-20，
  
  网络出版日期：2022-08-29，
  
  收稿日期：2022-04-19，
  
  录用日期：2022-05-24
- 稿件说明：
移动端阅览
王泽钜,绳新如,李光锋等.编织聚合物[J].高分子学报,2022,53(11):1301-1315.

Wang Ze-ju,Sheng Xin-ru,Li Guang-feng,et al.Woven Polymers[J].ACTA POLYMERICA SINICA,2022,53(11):1301-1315.
王泽钜,绳新如,李光锋等.编织聚合物[J].高分子学报,2022,53(11):1301-1315. DOI： 10.11777/j.issn1000-3304.2022.22130.

Wang Ze-ju,Sheng Xin-ru,Li Guang-feng,et al.Woven Polymers[J].ACTA POLYMERICA SINICA,2022,53(11):1301-1315. DOI： 10.11777/j.issn1000-3304.2022.22130.

摘要

编织聚合物是高分子科学与传统编织相结合的产物. 同普通聚合物材料相比，编织的经纬线程赋予了编织聚合物材料独特的网络拓扑以及丰富的力学性能. 但是，编织聚合物作为一类新兴的高分子材料，其在结构调控、性能探究以及应用拓展方面仍需进一步发展. 因此，本文从分子结出发，详细介绍了小分子打结的发展对于构建编织聚合物的推动作用；随后，总结了现有晶态编织聚合物以及柔性编织聚合物的构筑方法、性能研究以及相关的应用尝试；最后，指出了编织聚合物在当前发展阶段所面临的关键问题与挑战. 以期通过本文的概述，为推动编织聚合物领域的快速发展提供参考，也为新型功能高分子材料的研发提供新思路.

Abstract

From the earliest knots to

various contemporary fabrics with exquisite patterns

weaving has been throughout the entire history of human civilization. The highly ordered warp and weft threads synergistically endow the woven materials with unique topologies and rich mechanical properties. Inspired by this

researchers attempt to integrate the woven topologies into polymer science

and develop new polymeric materials with well-defined structures—woven polymers. Woven polymers are a kind of polymer networks constructed by cross-nodes as the basic units and cross-linking with each other

which are mainly divided into two categories: one is crystalline woven polymers

which possess long-range ordered molecular woven threads

mainly including metal organic frameworks (MOFs) and covalent organic frameworks (COFs)

etc

.; the other type is flexible woven polymers

which are generally unordered over long ranges

while the incorporation of woven crosslinks can significantly enhance the physical and chemical properties of the polymers

similar to what the macroscopic woven structures do. In the woven polymer networks

the dynamically woven cross-links can effectively dissociate to dissipate energy under external stimuli

giving the entire polymer networks excellent dynamicity and toughness. Meanwhile

the warp and weft threads can slip relatively after the dissociation of the dynamic site

so that the stress could be transmitted to the entire polymer network

and the strength and resilience of the network are improved while the stability of the weaving topology is maintained. Therefore

the woven polymers have broad application prospects in the construction of mechanically stable crystalline framework materials and new flexible functional polymer materials. However

as an emerging polymer material system

woven polymers still need further development in terms of structure optimization

performance exploration and application expansion. This review first focuses on the molecule knots

introducing various construction strategies in deta

il and expounding their vital roles in the development of woven polymers. Then

we summarize the construction methods

performance tests and related attempts on application of existing crystalline woven polymers and flexible woven polymers. Finally

the key scientific issues and challenges in the field of woven polymers are discussed and the future application prospects are prospected. It is firmly believed that woven polymers are a very bright field of research

possessing new and interesting aspects waiting to be explored and discovered. It is anticipated that this review will provide references and clear veins for the rapid development of woven polymers

and new approaches for the research of new functional polymer materials.

关键词

编织聚合物，分子结，编织框架材料，机械适应性，拓扑网络

Keywords

Woven polymersMolecular knotsWoven framework materialsMechanical adaptabilityTopology network

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