纳米纤维复合材料的离子传输动力学调控及其电化学应用

贾绪平; 李晓晓; 缪月娥; 刘天西

doi:10.11777/j.issn1000-3304.2024.24012

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纳米纤维复合材料的离子传输动力学调控及其电化学应用

专论 | 更新时间：2024-09-20

- 纳米纤维复合材料的离子传输动力学调控及其电化学应用
- Regulated Ion Transport Dynamics and Electrochemical Applications of Nanofiber Composites
- 高分子学报 2024年55卷第5期页码：509-531
- 作者机构：
  
  1.东华大学材料科学与工程学院纤维材料改性国家重点实验室上海 201620
  2.江南大学化学与材料工程学院合成与生物胶体教育部重点实验室无锡 214122
- 作者简介：
  
  [ "缪月娥，女，1987 年生. 2010年本科毕业于东南大学化学化工学院；2015年于复旦大学高分子科学系获博士学位；2016年至今先后任东华大学材料科学与工程学院讲师/副研究员/研究员. 纤维材料改性国家重点实验室固定成员. 2023 年获国家自然科学基金优秀青年科学基金资助. 2022年入选上海市青年科技启明星计划，主持了国家自然科学基金青年科学基金、面上项目、优秀青年科学基金等项目. 主要研究领域为高分子纳米纤维功能复合材料、新型电化学储能复合材料与技术." ]
- 基金信息：
  
  国家自然科学基金(基金号 ┣22075042);52322302┫
- DOI：10.11777/j.issn1000-3304.2024.24012
  中图分类号：
- 纸质出版日期：2024-05-20，
  
  网络出版日期：2024-03-18，
  
  收稿日期：2024-01-14，
  
  录用日期：2024-02-22
- 稿件说明：
移动端阅览
贾绪平, 李晓晓, 缪月娥, 刘天西. 纳米纤维复合材料的离子传输动力学调控及其电化学应用. 高分子学报, 2024, 55(5), 509-531

Jia, X. P.; Li, X. X.; Miao, Y. E.; Liu, T. X. Regulated ion transport dynamics and electrochemical applications of nanofiber composites. Acta Polymerica Sinica, 2024, 55(5), 509-531
贾绪平, 李晓晓, 缪月娥, 刘天西. 纳米纤维复合材料的离子传输动力学调控及其电化学应用. 高分子学报, 2024, 55(5), 509-531 DOI： 10.11777/j.issn1000-3304.2024.24012.

Jia, X. P.; Li, X. X.; Miao, Y. E.; Liu, T. X. Regulated ion transport dynamics and electrochemical applications of nanofiber composites. Acta Polymerica Sinica, 2024, 55(5), 509-531 DOI： 10.11777/j.issn1000-3304.2024.24012.

摘要

纳米纤维复合材料因具有高孔隙率、高比表面积以及多样化的组成和结构可设计性被广泛应用于锂硫电池、锂空电池等新型锂金属电池储能体系中. 电池的电化学性能主要依赖于充放电反应中的离子传输过程，而纳米纤维的结构形态以及表/界面性质对于离子传输动力学具有重要影响. 因此，本文针对新型储能电池应用中离子传输动力学缓慢、中间产物如多硫阴离子等易穿梭，以及负极枝晶生长等关键科学与技术问题，综述了纳米纤维复合材料的创新性设计和制备方法；进一步结合本课题组近期工作重点，阐述了纳米纤维复合材料的组成与结构调控对锂电池中离子传输动力学的优化作用；最后，总结了纳米纤维复合材料在锂电池正负极、隔膜、电解质等领域的应用进展，并讨论了其在新型储能设备领域的挑战和未来发展前景.

Abstract

Nanofiber composites have been widely used in new energy storage systems like lithium-metal batteries (LMBs

including lithium-sulfur batteries

lithium-air batteries

etc

.) due to their high porosity

high specific surface area

diversified compositions and structural designability. The electrochemical performance of the batteries largely depends on the ion transfer process during charging and discharging

while the structural morphology and surface/interface properties of nanofiber composites have an important influence on the ion transport kinetics in batteries. Therefore

focusing on the key scientific and technical issues of sluggish ion transport dynamics and the shuttling of intermediate lithium polysulfides faced by LMBs

this review firstly introduces different new designs and preparation methods of nanofiber composites. Then

the effects of composition and structure of nanofiber composites on the regulation and optimization of ion transport kinetics in lithium batteries are discussed in d

etail by combining the recent works of our team. Following

the applications of nanofiber composites in different fields of lithium batteries are summarized

such as anodes

cathodes

separators

and solid-state electrolytes

etc

. The challenges and prospects of nanofiber composites are finally proposed in future applications of high-performance energy storage equipment.

关键词

纳米纤维纳米复合材料静电纺丝离子传输动力学电化学性能

Keywords

NanofibersNanocompositesElectrospinningIon transport dynamicsElectrochemical performance

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