超96%近红外光隔热率的高性能半透明有机太阳能电池

李耀凯; 关诗陶; 李水兴; 左立见; 陈红征

doi:10.11777/j.issn1000-3304.2024.24102

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超96%近红外光隔热率的高性能半透明有机太阳能电池

研究论文 | 更新时间：2024-11-26

- 超96%近红外光隔热率的高性能半透明有机太阳能电池
- High-performance Semitransparent Organic Solar Cells Exceeding 96% Near-infrared Light Insulation Rate
- 高分子学报 2024年55卷第9期页码：1134-1144
- 作者机构：
  
  1.浙江大学硅及先进半导体材料全国重点实验室高分子科学与工程学系杭州 310027
  2.浙江大学杭州国际科创中心信息与功能材料研究院杭州 311200
- 作者简介：
  
  E-mail: hzchen@zju.edu.cn
- 基金信息：
  
  国家重点研发计划(2019YFA0705902)
- DOI：10.11777/j.issn1000-3304.2024.24102
  中图分类号：
- 纸质出版日期：2024-09-20，
  
  网络出版日期：2024-07-10，
  
  收稿日期：2024-04-06，
  
  录用日期：2024-05-06
- 稿件说明：
移动端阅览
李耀凯, 关诗陶, 李水兴, 左立见, 陈红征. 超96%近红外光隔热率的高性能半透明有机太阳能电池. 高分子学报, 2024, 55(9), 1134-1144

Li, Y. K.; Guan, S. T.; Li, S. X.; Zuo, L. J.; Chen, H. Z. High-performance semitransparent organic solar cells exceeding 96% near-infrared light insulation rate. Acta Polymerica Sinica, 2024, 55(9), 1134-1144
李耀凯, 关诗陶, 李水兴, 左立见, 陈红征. 超96%近红外光隔热率的高性能半透明有机太阳能电池. 高分子学报, 2024, 55(9), 1134-1144 DOI： 10.11777/j.issn1000-3304.2024.24102.

Li, Y. K.; Guan, S. T.; Li, S. X.; Zuo, L. J.; Chen, H. Z. High-performance semitransparent organic solar cells exceeding 96% near-infrared light insulation rate. Acta Polymerica Sinica, 2024, 55(9), 1134-1144 DOI： 10.11777/j.issn1000-3304.2024.24102.

摘要

半透明光伏是一种广受关注的太阳能光电转换技术，在吸光供能的同时，还可以保留一定的透光性. 但半透明有机太阳能电池(semitransparent organic solar cells，STOPV)要想实现应用，必须解决能量转换效率(power conversion efficiency，PCE)、可见光透过率(average photopic transmittance，APT)与近红外光隔热率(infrared-light rejection rate，IRR)有机统一的问题. 不同于传统的单一优化策略，本文工作通过采用高性能三元策略和多层光学调控层的方法来协同改善STOPV的性能. 材料层面，通过结合宽带隙给体和2个吸收相似但对称性不同的近红外受体分子，将单结三元不透明有机太阳能电池的效率优化至18.66%. 器件层面，提出三重光学调控方案，同时引入减反射层(anti-reflection layer，ARC)，二氧化碲(tellurium dioxide，TeO

)光学层和带通滤光片(bandpass filter，BF)，来优化器件的透光性. 最终制备的最佳STOPV，其PCE和APT分别达到了12.82%和35.70%，对应的光利用效率(light utilization efficiency，LUE)为4.6%，并且近红外光隔热率达到96.8%，实现了PCE、APT和IRR的均衡提升. 本文提出了一种开发设计高性能STOPV的有效方案，有利于进一步推动STOPV的商业化应用进展.

Abstract

Semitransparent organic solar cells (STOPV) are a widely acknowledged solar energy conversion technology that can simultaneously absorb invisible light for energy production while allowing visible light transmission for transparency. However

regarding STOPV integrated on building to reach practical application in the future

the harmonious unification of power conversion efficiency (PCE)

average photopic transmittance (APT)

and the infrared-light rejection rate (IRR) must be achieved. In contrast to traditional single-optimization strategies

we present an approach to enhancing STOPV performance by using a ternary strategy coupled with multiple optical modulation engineering. On the materials level

by combining the wide bandgap donor PM6 and two near-infrared acceptors owing similar absorption but different end groups combinations (symmetric molecule BTP-eC9 and asymmetric molecule BTP-S9)

we have optimized the efficiency of a single-junction ternary opaque organic solar cell to 18.66%. On the device level

we propose a triple optical manipulation method by integrating an anti-reflection layer (ARC)

a tellurium dioxide (TeO

) optical layer

and a bandpass filter (BF) into

the original STOPV structure

to address the see-saw effect among PCE

APT and IRR. Ultimately

our optimized STOPV achieved a PCE of 12.82% and APT of 35.70%

causing a light utilization efficiency (LUE) of 4.6%

and an infrared-light rejection rate of 96.8%

ranking one of the highest performance multifunction-STOPV.

关键词

半透明有机太阳能电池光学调控二氧化碲近红外光阻隔光电建筑集成

Keywords

Semitransparent organic solar cellsOptical manipulationTellurium dioxideNear-infrared light insulationPhotovoltaic building integration

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