附生结晶调控有机高分子半导体材料聚集态结构与性能

闫敬越; 刘玉敏; 黄华东; 高灿; 董焕丽; 李忠明

doi:10.11777/j.issn1000-3304.2024.24152

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附生结晶调控有机高分子半导体材料聚集态结构与性能

综述 | 更新时间：2024-12-24

- 附生结晶调控有机高分子半导体材料聚集态结构与性能
- Structure and Property Regulation of Polymer Semiconductors via Epitaxial Crystallization
- 高分子学报 2024年55卷第11期页码：1441-1462
- 作者机构：
  
  1.中国科学院化学研究所北京分子科学国家重点实验室北京 100190
  2.四川大学高分子科学与工程学院四川 610065
  3.中国科学院大学北京 100049
- 作者简介：
  
  [ "刘玉敏，女，1990年生. 2013年获天津理工大学学士学位；2021年获得天津大学化学工程博士学位，师从王静康院士和龚俊波教授，从事药物结晶研究. 2017~2019年，加入英国曼彻斯特大学晶体化学和粒子过程工程研究小组，与Roger Davey教授和Aurora Cruz Cabeza教授合作，开展晶体生长研究. 现在中国科学院化学研究所董焕丽研究员课题组从事博士后研究工作，主要集中在有机半导体晶体材料制备及其光电性能方面的研究." ]
  [ "高灿，女，1989年生，现任中国科学院化学研究所副研究员. 2012年，陕西师范大学获学士学位；2015年，中国科学院青海盐湖研究所获硕士学位；2019年，澳大利亚墨尔本大学获博士学位. 2020~2022年于中国科学院化学研究所开展博士后研究. 现任Wearable Electronics期刊执行编辑. 主要研究方向为有机发光晶体管材料与器件." ]
- 基金信息：
  
  中国科学院稳定支持基础研究领域青年团队计划(YSBR-053);国家自然科学基金(基金号 ┣52233010);22021002┫
- DOI：10.11777/j.issn1000-3304.2024.24152
  中图分类号：
- CSTR：32057.14.GFZXB.2024.7267
- 收稿日期：2024-05-27，
  
  录用日期：2024-06-28，
  
  网络出版日期：2024-09-24，
  
  纸质出版日期：2024-11-20
- 稿件说明：
移动端阅览
闫敬越, 刘玉敏, 黄华东, 高灿, 董焕丽, 李忠明. 附生结晶调控有机高分子半导体材料聚集态结构与性能. 高分子学报, 2024, 55(11), 1441-1462

Yan, J. Y.; Liu, Y. M.; Huang, H. D.; Gao, C; Dong, H. L.; Li, Z. M. Structure and property regulation of polymer semiconductors via epitaxial crystallization. Acta Polymerica Sinica, 2024, 55(11), 1441-1462
闫敬越, 刘玉敏, 黄华东, 高灿, 董焕丽, 李忠明. 附生结晶调控有机高分子半导体材料聚集态结构与性能. 高分子学报, 2024, 55(11), 1441-1462 DOI： 10.11777/j.issn1000-3304.2024.24152. CSTR： 32057.14.GFZXB.2024.7267.

Yan, J. Y.; Liu, Y. M.; Huang, H. D.; Gao, C; Dong, H. L.; Li, Z. M. Structure and property regulation of polymer semiconductors via epitaxial crystallization. Acta Polymerica Sinica, 2024, 55(11), 1441-1462 DOI： 10.11777/j.issn1000-3304.2024.24152. CSTR： 32057.14.GFZXB.2024.7267.

摘要

高质量共轭高分子半导体晶体材料的制备对于其基础物性的研究和高性能有机光电器件的构筑具有至关重要的意义. 但是高分子材料存在本征分子量大、呈分散性、链间易于缠结等特征，导致其高度有序共轭高分子聚集体的制备面临巨大挑战. 本文立足于有机高分子半导体材料聚集态结构与性能调控，在传统溶液组装策略的基础上，介绍了新型取向结晶策略，重点探讨了附生结晶的影响因素以及附生结晶在调控有机高分子半导体材料聚集态结构与性能方面的优势，并对目前附生结晶存在的问题进行了总结与展望.

Abstract

The field of organic electronics has made significant progress after more than 40 years of research

giving rise to a series of emerging related areas. Due to limitations such as limited conjugated size of small molecules and high degree of disorders in conjugated polymers

research in this field is currently facing performance limits and its development is distinctly hindered. The preparation of high-quality semiconductor crystals of conjugated polymers is of great significance for the study of their basic physical properties and the construction of organic optoelectronic devices with the high performance. However

due to the inherent characteristics such as high molecular weight

dispersibility

and easy entanglement between chains

the acquisition of highly ordered aggregates for conjugated polymers faces enormous challenges. Study on the crystallization of conjugated polymers is definitely important for preparing their high-quality crystals in order to overcome the current performance limitations in organic electronics

and would be expected to provide an important research platform for basic physical properties of conjugated polymers. Epitaxial crystallization is a surface-induced crystallization method. The existence of oriented substrate can reduce the nucleation barrier of crystallization processes and make the crystallization processes more easily to occur in comparison to the traditional solution crystallization. Therefore

epitaxial crystallization has become a common method for regulating the aggregation structure and properties of organic polymer semiconductor materials. In this contribution

we first briefly introduced the regulation of the aggregate structures of organic polymer semiconductor materials through traditional solution assembly and new oriented crystallization strategies. The factors of epitaxial crystallization and their advantages on regulating the aggregate structures and properties of organic polymer semiconductor materials were then particularly summarized. Future study on epitaxial crystallization in organic conjugated polymers was prospected in the end.

关键词

Keywords

references

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