基于氯菌酸自组装单分子层的大面积有机太阳能电池

郑颖聪; 严岑琪; 何韦; 李鸿祥; 龚钰扉; 胡颖玥; 王嘉宇; 薛启帆; 孙会靓; 孟磊; 李永舫; 程沛

doi:10.11777/j.issn1000-3304.2024.24312

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基于氯菌酸自组装单分子层的大面积有机太阳能电池

研究论文 | 更新时间：2025-07-08

- 基于氯菌酸自组装单分子层的大面积有机太阳能电池
- Large-area Organic Photovoltaics Based on Chlorendic Acid Self-assembled Monolayer
- 高分子学报 2025年56卷第7期页码：1088-1098
- 作者机构：
  
  1.四川大学高分子科学与工程学院先进高分子材料全国重点实验室成都 610065
  2.中国科学院化学研究所有机固体重点实验室北京 100190
  3.华南理工大学发光材料与器件国家重点实验室高分子光电材料与器件研究所广州 510640
  4.赣南师范大学化学化工学院赣州 341000
- 作者简介：
  
  E-mail: lihongxiang@scu.edu.cn
  chengpei@scu.edu.cn
- 基金信息：
  
  国家自然科学基金(基金号 ┣52403239);52403331┫;四川省科技计划项目(2023YFH0085;2023YFH0086;2023YFH0087);先进高分子材料全国重点实验室自主课题(基金号 sklpme 2023-2-11;sklpme 2024-2-15)
- DOI：10.11777/j.issn1000-3304.2024.24312
  中图分类号：
- CSTR：32057.14.GFZXB.2025.7349
- 收稿日期：2024-12-30，
  
  录用日期：2025-01-26，
  
  网络出版日期：2025-04-07，
  
  纸质出版日期：2025-07-20
- 稿件说明：
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郑颖聪, 严岑琪, 何韦, 李鸿祥, 龚钰扉, 胡颖玥, 王嘉宇, 薛启帆, 孙会靓, 孟磊, 李永舫, 程沛. 基于氯菌酸自组装单分子层的大面积有机太阳能电池. 高分子学报, 2025, 56(7), 1088-1098

Zheng, Y. C.; Yan, C. Q.; He, W.; Li, H. X.; Gong, Y. F.; Hu, Y. Y.; Wang, J. Y.; Xue, Q. F.; Sun, H. L.; Meng, L.; Li, Y. F.; Cheng, P. Large-area organic photovoltaics based on chlorendic acid self-assembled monolayer. Acta Polymerica Sinica, 2025, 56(7), 1088-1098
郑颖聪, 严岑琪, 何韦, 李鸿祥, 龚钰扉, 胡颖玥, 王嘉宇, 薛启帆, 孙会靓, 孟磊, 李永舫, 程沛. 基于氯菌酸自组装单分子层的大面积有机太阳能电池. 高分子学报, 2025, 56(7), 1088-1098 DOI： 10.11777/j.issn1000-3304.2024.24312. CSTR： 32057.14.GFZXB.2025.7349.

Zheng, Y. C.; Yan, C. Q.; He, W.; Li, H. X.; Gong, Y. F.; Hu, Y. Y.; Wang, J. Y.; Xue, Q. F.; Sun, H. L.; Meng, L.; Li, Y. F.; Cheng, P. Large-area organic photovoltaics based on chlorendic acid self-assembled monolayer. Acta Polymerica Sinica, 2025, 56(7), 1088-1098 DOI： 10.11777/j.issn1000-3304.2024.24312. CSTR： 32057.14.GFZXB.2025.7349.

摘要

采用氯菌酸小分子(6C2A)原位自组装作为有机太阳能电池(OPV)的阳极界面层(AIL)，并通过刮涂法制备了基于PM6:BTP-eC9活性层的二元单结正向OPV器件. 相较于传统PEDOT:PSS基器件(光电转换效率为17.6%，短路电流密度为27.0 mA·cm

-2

)，基于6C2A的器件展现出更高的光电转换效率(18.2%)和短路电流密度(27.7 mA·cm

-2

). 这一提升得益于6C2A阳极界面层增强了吸收，提高了激子解离效率，促进了载流子抽取，并抑制了载流子复合. 此外，2 cm

的6C2A基器件效率达到16.2%，优于PEDOT:PSS基器件(15.7%). 本研究通过自组装阳极界面层替代传统PEDOT:PSS，为有机太阳能电池的高通量、连续工业化生产提供了新思路.

Abstract

In order to fulfill the requirements of future industrialization

organic photovoltaics (OPVs) necessitate improved power conversion efficiency (PCE) and optimized manufacturing processes. Anode interfacial layer (AIL) constitutes a vital element within the OPV structure.However

the most widely used PEDOT:PSS anode interficial layer exhibits hygroscopic and acidic nature

which compromise the stability of the device. Herein

this study employs chlorendic acid small molecule

in situ

sel

f-assembly as the anode interfacial layer for organic photovoltaics and fabricates binary single-junction forward OPV devices based on the PM6:BTP-eC9 active layer using the blade coating method. Compared to traditional PEDOT:PSS-based devices (with a photoelectric conversion efficiency of 17.6% and a short-circuit current density of 27.0 mA·cm

-2

devices based on 6C2A exhibit higher photoelectric conversion efficiency (18.2%) and short-circuit current density (27.7 mA·cm

-2

). This enhancement is attributed to the 6C2A anode interfacial layer

which strengthens absorption

improves exciton dissociation efficiency

facilitates charge carrier extraction

and suppresses charge carrier recombination. Also

the 6C2A anode interficial layer shows great stability when exposed to air of 25% relative humidity

overcoming the hygroscopicity of traditional PEDOT:PSS. Furthermore

the efficiency of the 6C2A-based devices with an area of 2 cm

reaches 16.2%

outperforming PEDOT:PSS-based devices (15.7%).The

in situ

self-assembly fabrication method can simplyfing the technique of production

streamlining manufacturing

reducing costs

and enhancing scalability. This study provides a new approach for the high-throughput

continuous industrial production of organic solar cells by substituting traditional PEDOT:PSS with self-assembled anode interficial layer.

关键词

Keywords

references

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