废塑料升级化学回收制备金属-有机框架材料

温雪莹; 冯玲玲; 戴郅焜; 胡桂新; 牛冉; 龚江

doi:10.11777/j.issn1000-3304.2026.26162

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废塑料升级化学回收制备金属-有机框架材料

综述 | 更新时间：2026-07-24

- 废塑料升级化学回收制备金属-有机框架材料
- Upcycling of Waste Plastics into Metal-Organic Frameworks via Chemical Recycling
- 高分子学报 2026年页码：1-27
- 作者机构：
  
  华中科技大学化学与化工学院能量转换与存储材料化学教育部重点实验室材料化学与服役失效湖北省重点实验室武汉 430074
- 作者简介：
  
  龚江，男，1988年生，华中科技大学化学与化工学院，研究员、博士生导师. 2010年于四川大学获高分子材料与工程学士学位，2015年于中国科学院长春应用化学研究所获高分子化学与物理博士学位，2015~2017年于德国马克斯-普朗克胶体界面研究所从事博士后研究，2017~2018年于美国得克萨斯州大学圣安东尼奥分校从事博士后研究，2018年10月加入华中科技大学化学与化工学院. 主要从事废弃塑料升级化学回收制备金属-有机框架(MOF)材料和碳材料，MOF材料的绿色合成与产业化应用，太阳能界面水蒸发与集成应用，在Progress in Polymer Science等期刊发表论文188篇，被引用超过1.07万次，申请专利60项，其中授权30项. 主持国家自然科学基金项目和企业横向项目十余项.
- 基金信息：
  
  国家自然科学基金(基金号 52373099)
- DOI：10.11777/j.issn1000-3304.2026.26162
  中图分类号：
- CSTR：32057.14.GFZXB.2026.7665
- 收稿：2026-05-09，
  
  录用：2026-06-11，
  
  网络首发：2026-07-24，
- 稿件说明：
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温雪莹, 冯玲玲, 戴郅焜, 胡桂新, 牛冉, 龚江. 废塑料升级化学回收制备金属-有机框架材料. 高分子学报, doi: 10.11777/j.issn1000-3304.2026.26162.

Wen, X. Y.; Feng, L. L.; Dai, Z. K.; Hu, G. X.; Niu, R.; Gong, J. Upcycling of waste plastics into metal-organic frameworks via chemical recycling. Acta Polymerica Sinica (in Chinese), doi: 10.11777/j.issn1000-3304.2026.26162.
温雪莹, 冯玲玲, 戴郅焜, 胡桂新, 牛冉, 龚江. 废塑料升级化学回收制备金属-有机框架材料. 高分子学报, doi: 10.11777/j.issn1000-3304.2026.26162. DOI： CSTR： 32057.14.GFZXB.2026.7665.

Wen, X. Y.; Feng, L. L.; Dai, Z. K.; Hu, G. X.; Niu, R.; Gong, J. Upcycling of waste plastics into metal-organic frameworks via chemical recycling. Acta Polymerica Sinica (in Chinese), doi: 10.11777/j.issn1000-3304.2026.26162. DOI： CSTR： 32057.14.GFZXB.2026.7665.

摘要

塑料污染对生态环境与人体健康构成重大威胁，发展高效绿色的废塑料回收利用技术迫在眉睫. 升级化学回收可将废塑料定向转化为高附加值化学品或功能材料，被认为是实现循环经济的关键路径. 金属-有机框架(MOF)材料因具有高比表面积、可调孔径和丰富活性位点成为极具潜力的功能性材料. 以废塑料作为配体前驱体，通过化学解聚获得有机酸并用于合成MOF，既能降低合成成本，又能实现废塑料的高值化资源化利用. 本文综述了近年来废塑料升级回收为MOF材料的研究进展，总结了各种合成策略，并介绍了制备的MOF在吸附、界面水蒸发以及能源存储与转换领域的应用. 最后，对当前面临的挑战及未来发展方向进行了分析与展望，以期为废塑料资源化与高性能MOF材料合成的协同发展提供参考.

Abstract

Plastic pollution poses a significant threat to the ecological environment and human health

making it urgent to develop efficient and green recycling technologies for waste plastics. Chemical upcycling

which can directionally convert waste plastics into high-value chemicals or functional materials

is considered a key pathway toward a circular economy. Metal-organic frameworks (MOFs) have emerged as highly promising functional materials due to their high specific surface area

tunable pore size

and abundant active sites. Using waste plastics as ligand precursors to obtain organic acids

via

chemical depolymerization for MOF synthesis not only reduces the synthesis cost but also enables high-value resource utilization of waste plastics. This article systematically reviews the recent research progress on upcycling waste plastics into MOF materials

summarizes various synthesis strategies

and presents the applications of the as-prepared MOFs in adsorption

interfacial water evaporation

and energy storage and conversion. Finally

the current challenges and future development directions are analyzed and prospected

aiming to provide a reference for the synergistic development of waste plastic valorization and the synthesis of high-performance MOF materials.

关键词

Keywords

references

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